International Journal of Basic and Applied Biology
Print ISSN: 2394-5820, Online ISSN: 2349-2539, Volume 2, Number 6; July-September, 2015, pp. 364-367
© Krishi Sanskriti Publications
http://www.krishisanskriti.org/ijbab.html
Characterization of Fibrous Scaffold using
Quantitative Nano-Mechanical Mapping
Mode of Atomic Force Microscope
Mohammad A. Hussain
1
, Adnan Memic
2
, Nazeeh S. Alothmani
3
, Rabah W. Al-dhaheri
4
,
Faten Al-hazmi
5
, Hani A. Alhadrami
6
and Ali Khademhosseini
7
1,2,3,4,5,6
KAU, Jeddah, KSA
7
Harvard-MIT, USA
E-mail:
1
mhussain2@kau.edu.sa,
2
amemic@kau.edu.sa,
3
nothmany@kau.edu.sa,
4
raldhaheri@kau.edu.sa,
5
fialhazmi@kau.edu.sa,
6
hanialhadrami@kau.edu.sa,
7
khademh@gmail.com,
Abstract—Electrospun polymeric fibers with nano and submicron
diameters amalgamated with inorganic nanoparticles, in particular,
those constructed with uniform reinforcements can be used as
scaffolds in tissue engineering. Importantly it warrants a
characterization of their mechanical properties particularly at the
nanoscale. The PeakForce Quantitative NanoMechanics (PF-QNM)
AFM mode allows to probe nanomechanical properties of the
material namely, DMT modulus, adhesion, dissipation and
deformation, at the same time along with topographical imaging. In
this paper we present results of PF-QNM characterization of three
kinds of electrospun nanofibers made from a 1:1 blend of two
polymers: PCL and PMMA with further addition of inorganic
nanoparticles (Ag and ZnO) at three ratios thereby adding another
degree of nanocomposition to the resulting nanocompoite nanofiber
scaffold. The results showed the inorganic nanoparticles Ag and
ZnO, with different shapes and sizes, appearing at the surface of the
nanofibers. Heterogeneous Ag and ZnO nanoparticle distribution
was observed on the nano fiber mesh. The Ag and ZnO contents were
different at different locations along the nanofibers lengths based on
their ratios in three different types of nanofiber mesh. The different
ratios of Ag:ZnO inorganic nanoparticles affected the DMT Modulus
as well as hydrophilic nature of the three kinds of nanofiber surfaces.
Increasing ZnO amount increased both the hardness and water
contact angle of the nanofiber mesh. For the same increase in the
(Ag:ZnO) ratio, ZnO doubled the %increase in hydrophobicity as
compared to Ag. From Ag:ZnO (30:30) to (100:30) increased the
water contact angle by 8% while altering the ratio (30:100)
increased it by 16%. The average DMT modulus was 0.62 ± 0.26
MPa for control mesh, 2.22 ± 0.61 MPa for Ag:ZnO (30:30), 5.62 ±
1.39 MPa for Ag:ZnO (100:30), and 63.87 ± 81.82 MPa for Ag:ZnO
(30:100) mesh.
1. INTRODUCTION
The last decade has seen an increasing trend in designing
scaffolds for tissue engineering from biodegradable polymeric
fibers with nano and submicron diameters specifically
produced by electrospinning method. Partly successes in using
such scaffolds are attributable to structural similarity to the
extracellular matrix (ECM), convenient porosity for cellular
proliferation, high surface area to volume ratio, reduced
immunogenicity and biodegradability among others [1]. After
implantation of such scaffolds, in biomechanical environment
of the body, however the fibers in the scaffolds are subjected
to stresses and strains in physiological conditions, thereby
standing a chance to permanent deformation or even failure to
scaffold structure. Therefore, there is a pressing need to
characterize their mechanical properties, especially at the
nanoscale as well as to assess resulting surface properties such
as wettability.
1.1 Nano-mechanical properties.
Atomic force microscopy (AFM) in the family of scanning
probe microscopy has emerged as a promising tool with a host
of powerful techniques that have been employed in imaging of
the components of biomaterials scaffolds and probing selected
mechanical properties under physiological conditions [2-4].
The PeakForce Quantitative NanoMechanics (PF-QNM) is
relatively a new addition to the host of techniques allowing to
measure nano-mechanical properties of the materials including
reduced Young`s modulus, adhesion, dissipation, and
deformation concurrently with topographical height imaging
[5].
1.2 Wettability.
Wettability pertains to the interaction between solid and fluid
phases at the interface. Strictly the contact angle of the fluid
with the solid phase at which the liquid–vapor interface meets
the solid–liquid interface, explains the wettability. This in turn
is determined by a force balance between adhesive and
cohesive forces. An increasing tendency of a drop to spread
out over a flat, decreases the contact angle, thereby providing
an inverse measure of wettability. A contact angle less than
90° (low contact angle) usually indicates that wetting of the