S1
Clickable UTP Analog for the Posttranscriptional Chemical Labeling and
Imaging of RNA
Anupam A. Sawant, Progya P. Mukherjee, Rahul K. Jangid,
Sanjeev Galande* and Seergazhi G. Srivatsan*
Electronic Supplementary Information
Contents Page
1. Materials S2
2. Instrumentation S2
3. Synthesis S3
Scheme S1. Synthesis of azide substrates 5 and 9 for CuAAC reactions S3
Fig. S1 Phosphorimage of transcription products obtained from reactions with
alkyne- modified UTP 3
S5
Fig. S2 PAGE of in vitro transcription reaction performed in presence of template T2 S6
Fig. S3 MALDI-TOF mass spectrum of alkyne-modified oligoribonucleotide
transcripts 4
S7
Table S1 Yield and mass data of alkyne-modified RNA transcript 4 and 10 S7
4. Enzymatic digestion of RNA ON 4 S7
Fig. S4 HPLC chromatogram of enzymatic digestion of RNA ON 4 S8
Fig S5 UV-thermal melting of control unmodified duplex and alkyne-modified
duplex
S9
5. In vitro transcription with plasmid DNA template in the presence of 3 S9
Fig. S6 HPLC chromatogram of ribonucleoside products obtained from enzymatic
digestion reactions of longer modified RNA transcripts containing 2
S10
6. Reverse transcription of alkyne-modified RNA transcripts containing 2 S10
Fig. S7 PCR amplified template sequence from pEGFPC1 vector used in
transcription reactions
S12
Fig. S8 Representative sequence alignment (BLAST) of PCR amplified DNA
products
S12
Table S2. Yield and mass data of posttranscriptionally functionalized RNA ONs 4
and 10
S13
Fig. S9 Posttranscriptional chemical modification of EU-modified RNA ON 10 by
CuAAC reaction
S14
Fig. S10 Posttranscriptional chemical modification of 59mer ODU-RNA by CuAAC
reaction using Alexa594-azide 6
S15
Fig. S11 Incorporation of ODU 2 into cellar RNA transcripts as detected by CuAAC
reactions using Alexa594-azide 6.
S15
Fig. S12 Quantification plots showing percentage of labeled nuclei by click reaction S16
Electronic Supplementary Material (ESI) for Organic & Biomolecular Chemistry.
This journal is © The Royal Society of Chemistry 2016