538 Journal of Crystal Growth 71 (1985) 538-550
North-Holland, Amsterdam
THE GROWTH OF GaSb UNDER MICROGRAVITY CONDITIONS
E. LENDVAY, M. HA,RSY, T. G()R()G, I. GYUR0, I. POZSGAI and F. KOLTAI
Research Institute for Technical Physics. Hungarian Acadern~, of Sciences. Budapest. Hungary
J. GYULAI, T. LOHNER, G. MEZEY, E. KOTAI and F. P,A, SZTI
Central Research Institute for Physics. Hungarian Academy of Sciences, Budapest, Hungary
and
V.T. HRJAPOV, N.A. KULTCHISKY and L.L. REGEL
Research Institute for Cosmic Investigations. Moscow. USSR
Received 5 April 1984; Manuscript received in final form 4 March 1985
A high quality GaSb bicrystal was grown in a Bridgman type arrangement under microgravity conditions on board of Salyut-6.
Rutherford back-scattering measurements indicate oxide and damage free surfaces. Scanning Electron Microscopy revealed micro-
facets on the space grown sample. The morphology of the sample suggests a crystallization quite free of a wall effect. A comparison is
given between space and terrestrial GaSb ingots, showing differences in surface quality, crystal perfection and hole mobilities. In the
space grown sample a l% ~ 2700 cm2 v-1 s-1 value was found while for the terrestrial control this value was only 2000 cm2 v-1 s-1
1. Introduction
Binary Am B v compounds are important materi-
als for optoelectric applications. To date lasers,
detectors and solar cells have been fabricated using
these semiconductors. GaSb, with a direct band
gap of 0.74 eV, is a very attractive material for
optoelectronic devices. Under conditions currently
used for growth it has a p-type conductivity without
intentional doping. However, bipolar conductivity
can also be achieved using different dopants, such
as Sn, Te or Zn [1-4]. More recently the develop-
ment of very high quantum efficiency GaSb pho-
todetectors in the 1.3-1.7 nm region have been
reported [3-5]. GaSb substrates are also used for
A1GaSb, GaAsSb, InGaAsSb and GaA1AsSb de-
tectors, LEDs and laser devices.
For these applications damage and inhomo-
geneity free crystals of high quality with low dislo-
cation densities are needed. Numerous publica-
tions describing different growth methods and
aimed to improve the quality of GaSb crystals
have been recently published, but the obtained
materials often contain macroscopic and micro-
scopic defects. Twins, for instance, can be easily
formed and also microfaceted growth is frequently
observed [6,7].GaSb is an ideal model for space
technology. Among the semiconductors it has a
relatively low melting point. Growing crystals un-
der microgravity conditions is not an energy con-
suming process. Investigating the GaSb crystals
grown both the macroscopic and microscopic
growth mechanisms could be studied examining
the crystal (defect) structure and morphology, as
well as the semiconductor properties. Microscopic
inhomogeneities associated with changes in the
growth rate respond very sensitively to the convec-
tion and the mechanical vibrations of the growth
system [8,9]. In order to study these effects in
detail, GaSb growth experiments were performed
during the first Soviet-Hungarian Space Flight on
board of Salyut-6, under microgravity conditions,
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