African Journal of Microbiology Research Vol. 7(3), pp. 202-210, 15 January, 2013
Available online at http://www.academicjournals.org/AJMR
DOI: 10.5897/AJMR12.1774
ISSN 1996-0808 ©2013 Academic Journals
Full Length Research Paper
DNA-binding activity and in vivo cytotoxicity of
Ganoderma applanatum (Pers.) Pat. supercritical-CO
2
extracts
Zeus S. Elumba
1
, Franco G. Teves
2
* and Roberto M. Malaluan
3
1
Department of Biology, Central Mindanao University, Musuan, Bukidnon, Philippines.
2
Department of Biological Sciences, Mindanao State University-Iligan Institute of Technology, Iligan City, Philippines.
3
Department of Chemical Engineering Technology, Mindanao State University-Iligan Institute of Technology,
Iligan City, Philippines.
Accepted 11 October, 2012
Ganoderma applanatum (Pers.) Pat. is a perennial and abundant mushroom in Bukidnon Province,
Philippines but its bioactivities have just been investigated lately. In this study, three supercritical-CO
2
(SC-CO
2
) extracts (GA1, GA2 and GA3) from the local strain of G. applanatum (Pers.) Pat. were examined
for their DNA-binding potential by means of biomolecular-chemical screening and in vivo cytotoxicity
using brine shrimp lethality assay (BSLA). All extracts contained secondary metabolites that have DNA-
binding activity towards salmon sperm DNA (Rf
2
/Rf
1
-ratio <1). For BSLA, the LC
50
(24 h) values ranged
from 177.82 to 354.81 μg/ml, indicating that the extracts are biologically active but with no significant
cytotoxicity. Reverse-phase HPLC and FT-IR spectroscopy were carried out to partially characterize the
extracts. Results of this study showed that G. applanatum (Pers.) Pat. from Bukidnon Province,
Philippines is a potential source of biologically active, non-toxic compounds with DNA-binding activity.
Key words: Ganoderma applanatum, DNA-binding activity, cytotoxicity, supercritical-CO
2
.
INTRODUCTION
Mushrooms have been valued for generations as source
of medicines or as food. For centuries, the medicinal use
of mushrooms such as Ganoderma was recorded in
China, Japan and Korea (Paterson, 2001). Of the
approximately 10,000 known species of mushrooms,
2000 are safe for human health and about 300 of them
possess medicinal properties (Wasser and Weis, 1999).
Mushrooms can synthesize a dazzling array of
biologically-active products which have no significant role
in their primary physiological processes (Kidukuli et al.,
2010). These are secondary metabolites that have often
attracted interest because of their biological effect on
other organisms. The strong activities of these bioactive
compounds enable mushrooms to survive in their
*Corresponding author. E-mail: franco_teves@yahoo.com.
Tel/Fax: (+63) 063 223 2343.
environments and allow them to out-compete their
environmental competitors (Kidukuli et al., 2010). It is not
surprising therefore that mushrooms contain secondary
metabolites that may have economic and pharmaceutical
values.
Ganoderma is a prolific producer of novel
“mycochemicals” (Paterson, 2006). There are reports on
its folkloric use for the treatment of various ailments
(Rowan et al., 2002; Jeong et al., 2008). Phytochemical
studies of Ganoderma applanatum (Pers.) Pat. showed
that it contains triterpenoids, tannins, sterols, steroids,
proteins and polysaccharides (Boh et al., 2000; de Silva
et al., 2006; Chairul et al., 1991; Strigina et al., 1971).
Previous studies demonstrated its antioxidant,
antimicrobial, immunomodulating, aldose reductase
inhibitors, nitric oxide synthase activators and anti-tumor
properties (Barranco et al., 2010; Muhsin et al., 2011;
Smania et al., 1999; Lee et al., 2005; Acharya et al.,
2005; Jeong et al., 2008; Chairul et al., 1991). However,