The 4th International Protein Kinases
in Drug Discovery & Development
meeting (October 20–22, 2003,
Philadelphia, USA) organized by SRI
(http://www.srinstitute.com) integrated
sessions that aimed to address the key
issues for kinase drug discovery. With
over 500 kinases in the human kinome
[1] and the costs of drug development
approaching the billion dollar mark,
the meeting focused on strategies to
move kinase drug discovery forward
in a more rapid and efficient manner,
including protein kinase target
validation, selectivity and drugability.
Topics included kinase assay technology
and profiling, novel strategies for kinase
inhibitor generation and associated
technologies for target identification and
validation, including RNAi applications.
Biochemical, cell-based assays
and screening methods
Owing to enormous efforts made within
the pharmaceutical industry, there are
now numerous biochemical and
cell-based screening methods for the
thorough profiling of kinase inhibitors.
Numerous factors such as cost, data
quality, throughput and screening-library
size need to be taken into consideration
and different assays can therefore yield
different screening results. Over 13 novel
assay formats were outlined during the
course of the meeting for tyrosine and
serine/threonine kinases, all with the
aim of resolving assay development
bottlenecks. Gregory Moore (Upstate
Discovery; http://www.upstate.com)
described assay formats for a range of
serine/threonine kinases using
monoclonal antibodies based on a small
collection of substrates and generic
fluorescent polarization assays for
tyrosine kinases based on Upstate’s
anti-phosphotyrosine antibody, 4G10.
Upstate currently has the capacity to
screen over 120 human protein kinases.
Michael Curtin (Promega Corporation;
http://www.promega.com) described
the development of two novel
homogeneous, non-radioactive high-
throughput assays to determine the
activity of many protein kinases These
assays can be readily optimized and
data were presented to demonstrate that
these formats can produce comparable
IC50s to those in the literature for
known inhibitors of protein kinase A
(PKA) and src family tyrosine kinases.
Phosphorylation of serine, threonine
and tyrosine residues is recognised as a
key mode of signal transduction and
amplification in eukaryotic cells. Pierre
Thibault (Caprion Pharmaceuticals;
http://www.caprion.com) described
how, with protein expression profiling as
a principle focus in proteomic research
for cancer therapies and biomarkers,
Caprion has pioneered a novel mass
spectrometry–bioinformatics approach
to measure relative protein abundance
from purified protein extracts of patient-
matched disease and normal specimens.
Steven Pelech (Kinexus Bioinformatics;
http://www.kinexus.ca) gave an
insightful overview of Kinexus’s antibody-
based detection method (Kinetworks™),
used to track >100 protein kinases
simultaneously in diverse cell and tissue
types. The multi-immunoblotting services
provided by Kinexus allows researchers to
accurately measure protein expression,
phosphorylation and interactions with
many other proteins through the direct
capture and quantification of proteins
by immobilized peptide probes.
Brian Holaway (Roche Protein
Expression Group; http://www.roche.com)
described the expression of p38 alpha
in inactive or activated forms using a
continuous-exchange cell-free (CECF)
protein expression system, which
potentially overcomes the limitations of
current cell-based methods. Rigorous
biophysical characterization, including
2D-NMR approaches, also identified a
number of conformational differences
between the activation states that
could potentially be exploited by
small-molecule inhibitors.
Structure-based design strategies
and applications
Structure-based drug design (SBDD)
facilitates rapid compound potency
optimization against protein targets.
Kinases are readily amenable to SBDD
and with >40 novel kinase structures
deposited in the Protein Data Bank,
there is a growing understanding of
how to achieve selectivity. Kumkum
Saxena (Vertex Pharmaceuticals;
http://www.vpharm.com) discussed
how rapid structure determination of
kinase target crystal structures is a key
tool in the drug discovery process at
Vertex. Many hundreds of constructs for
each kinase are designed, expressed and
purified by high-throughput methods
and, following rigorous protein analysis,
this approach produces a large increase
in crystallization success rates of these
update conference DDT Vol. 9, No. 1 January 2004
1359-6446/04/$ – see front matter ©2004 Elsevier Ltd. All rights reserved. PII: S1359-6446(03)02932-5 16 www.drugdiscoverytoday.com
Protein kinases in drug discovery
and development
Adrian Gill, Department of Medicinal Chemistry, Astex Technology, 436 Cambridge Science Park, Milton Road, Cambridge, CB4 0WE,
e-mail: a.gill@astex-technology.com