separations
Article
Automated Screening and Filtering Scripts for
GC×GC-TOFMS Metabolomics Data
Seo Lin Nam , A. Paulina de la Mata and James J. Harynuk *
Citation: Nam, S.L.; de la Mata, A.P.;
Harynuk, J.J. Automated Screening
and Filtering Scripts for
GC×GC-TOFMS Metabolomics Data.
Separations 2021, 8, 84. https://
doi.org/10.3390/separations8060084
Academic Editor: Alena Kubatova
Received: 18 May 2021
Accepted: 10 June 2021
Published: 15 June 2021
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Department of Chemistry, University of Alberta, 11227 Saskatchewan Drive, Edmonton, AB T6G 2G2, Canada;
seolin@ualberta.ca (S.L.N.); delamata@ualberta.ca (A.P.d.l.M.)
* Correspondence: james.harynuk@ualberta.ca; Tel.: +1-780-492-8303; Fax: +1-780-492-8231
Abstract: Comprehensive two-dimensional gas chromatography mass spectrometry (GC×GC-MS)
is a powerful tool for the analysis of complex mixtures, and it is ideally suited to discovery studies
where the entire sample is potentially of interest. Unfortunately, when unit mass resolution mass
spectrometers are used, many detected compounds have spectra that do not match well with
libraries. This could be due to the compound not being in the library, or the compound having a
weak/nonexistent molecular ion cluster. While high-speed, high-resolution mass spectrometers,
or ion sources with softer ionization than 70 eV electron impact (EI) may help with some of this,
many GC×GC systems presently in use employ low-resolution mass spectrometers and 70 eV EI
ionization. Scripting tools that apply filters to GC×GC-TOFMS data based on logical operations
applied to spectral and/or retention data have been used previously for environmental and petroleum
samples. This approach rapidly filters GC×GC-TOFMS peak tables (or raw data) and is available
in software from multiple vendors. In this work, we present a series of scripts that have been
developed to rapidly classify major groups of compounds that are of relevance to metabolomics
studies including: fatty acid methyl esters, free fatty acids, aldehydes, alcohols, ketones, amino acids,
and carbohydrates.
Keywords: comprehensive two-dimensional gas chromatography-mass spectrometry (GC×GC-MS);
scripting; metabolomics; data analysis; data visualization
1. Introduction
Most of the GC-based metabolomics applications combine GC with MS detection to
help with the identification of unknown analytes. Metabolomics samples typically exhibit
high complexity due to their diverse chemical content that is present at wide concentration
ranges. In non-target studies, accurate identification of metabolites at low concentrations
can be complicated by coelutions and/or peak distortion due to closely/coeluting highly
abundant metabolites [1,2]. Low-concentration analytes can also be easily obscured due to
noise in the spectrum that can hinder the qualitative identification of peaks based on mass
spectral library matching. Meanwhile, overloaded peaks from high-concentration species
may lead to inaccurate identification arising from detector saturation and distortion of
mass spectra [3].
As a platform, comprehensive two-dimensional gas chromatography time-of-flight
mass spectrometry (GC×GC-TOFMS) is an excellent tool for non-target metabolomics.
The higher and more effective use of peak capacity when compared to one-dimensional
GC methods, results in improved signal-to-noise ratios due to increased signal (focus-
ing/band compression at modulator) and decreased noise (separation of analytes from
primary column bleed and coeluting analytes). Consequently, spectra are cleaner, allowing
improved compound identification. When compared to LC-MS methods, matrix effects are
less in GC-MS, and the technique offers a broad dynamic range [4]. Additionally, GC×GC
techniques provide chromatograms with an inherently ordered structure, which is useful
for the identification of unknown compounds. Moreover, this technique is advantageous
Separations 2021, 8, 84. https://doi.org/10.3390/separations8060084 https://www.mdpi.com/journal/separations