1
Facile tuning of plasmon bands in hollow silver nanoshells using
mild reductant and mild stabilizer
Satarupa Pattanayak
a
, Amiya Priyam
a,
* and Pradip Paik
b,c
Supplementary Information
Optimization of synthesis temperature
Figure S1. The effect of synthesis temperature on the UV-Vis spectra of silver nanoparticles prepared by
reduction of Ag
2
O NPs at basic pH. (Stabilizer : citrate; Reducing agent :hydrazine hydrate)
The reduction of Ag
2
O NPs was carried out at different temperatures using hydrazine hydrate as
reducing agent. In this experiment, there are two oppositely moving ‘diffusion-reaction’ fronts and
the temperature at which the both become comparable to each other, hollow structures are likely to be
formed. Spectroscopically, the formation of hollow plasmonic nanostructures is indicated by the red-
shift in the plasmon peak. The SPR peak is observed at 409 nm for the syntheses at 10
o
C, 15
o
C and
25
o
C. But, the peak red-shifts to 423 nm at 20
o
C. As the maximum redshift is observed at 20
o
C, this
is chosen as the synthesis temperature for rest of the experiments.
Electronic Supplementary Material (ESI) for Dalton Transactions
This journal is © The Royal Society of Chemistry 2013