Journal of Atmospheric Chemistry 38: 195–227, 2001.
© 2001 Kluwer Academic Publishers. Printed in the Netherlands.
195
Formulation and Evaluation of IMS, an Interactive
Three-Dimensional Tropospheric Chemical
Transport Model 1. Model Emission Schemes
and Transport Processes
⋆
K.-Y. WANG
1
, J. A. PYLE
1
and D. E. SHALLCROSS
1,2
1
Centre for Atmospheric Science, Cambridge University, CB2 1EW, U.K.
2
School of Chemistry, University of Bristol, BS8 1TS, U.K.
(Received: 1 May 2000; in final form: 16 June 2000)
Abstract. In part one of this series of papers on a new integrated modelling system (IMS), the
interactive three-dimensional chemical transport model (CTM), we present a detailed description of
the interactive emission scheme for biogenic species and outline the datasets used for anthropogenic
species. In addition, we describe the transport scheme employed in this model. The biogenic emission
schemes incorporate the high-resolution Olson World Ecosystem data (Olson, 1992), the satellite-
sensed terrestrial vegetation data from AVHRR (A Very High Resolution Radiometer) (Brown et
al., 1985), and the CZCS (Coastal Zone Color Scanner) data (Erickson and Eaton, 1993). These
datasets provide seasonal variations in surface biogenic emissions. The emission schemes are tested
against other estimates (e.g., GEIA) and equilibrium emissions. A comparison of terrestrial biogenic
fluxes, both the spatial and temporal (seasonal) variation of modelled surface net primary produc-
tion, is consistent with the geographical variations of the global vegetation index (GVI) distribution
derived from AVHRR. The annual net primary production is 76000 Tg C yr
−1
, which compares well
with the 40500–78000 Tg C yr
−1
estimated by Melillo et al. (1993). This indicates that the model
works well in capturing spatial and seasonal variations in the terrestrial vegetation. The modelled
surface vegetation fluxes are verified against data from Guenther et al. (1995). While the comparison
shows a generally good agreement in terms of the temporal and spatial distributions of isoprene
(530 Tg yr
−1
), large discrepancies are seen over the tropical locations which often exhibit strong
seasonality in rainfall and very small variation in temperature. These differences indicate that a
large difference in the estimation between an empirical relation and an LSM calculation occurs if
an area in which seasonal distribution of rainfall is the main factor which determines the type of
vegetation. In this paper, we assess (results are discussed in following papers) the role of changing
surface biogenic distributions in surface-to-atmosphere biogenic fluxes (both ocean-to-atmosphere
and land-to-atmosphere).
Key words: CTM, LSM, emissions, transport.
⋆
This article is related to another in Volume 38, issue 1, pages 31–71, ‘Formulation and Evalu-
ation of IMS, an Interactive Three Dimensional Tropospheric Chemical Transport Model 2. Model
Chemistry and Comparison of Modelled CH
4
, CO, and O
3
with Surface Measurements’, by K.-Y.
Wang, J. A. Pyle, D. E. Shallcross, and D. J. Larry.