catalysts
Review
Catalytic Membrane Reactors: The Industrial
Applications Perspective
Catia Algieri
1,
*, Gerardo Coppola
2
, Debolina Mukherjee
2
, Mahaad Issa Shammas
3
, Vincenza Calabro
2
,
Stefano Curcio
2
and Sudip Chakraborty
2,
*
Citation: Algieri, C.; Coppola, G.;
Mukherjee, D.; Shammas, M.I.;
Calabro, V.; Curcio, S.; Chakraborty, S.
Catalytic Membrane Reactors:
The Industrial Applications
Perspective. Catalysts 2021, 11, 691.
https://doi.org/10.3390/
catal11060691
Academic Editor: Jose Antonio
Calles Martín
Received: 23 April 2021
Accepted: 27 May 2021
Published: 29 May 2021
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4.0/).
1
Institute on Membrane Technology, National Research Council of Italy (ITM–CNR), Cubo 17C,
Via Pietro Bucci, 87036 Rende, Italy
2
Department of DIMES, University of Calabria, Via Pietro Bucci, Cubo 42A, 87036 Rende, Italy;
coppola0gerardo@gmail.com (G.C.); DEBOLINA.MUKHERJEE@unical.it (D.M.);
vincenza.calabro@unical.it (V.C.); stefano.curcio@unical.it (S.C.)
3
Department of Civil & Environmental Engineering at Dhofar University, Salalah 211, Sultanate of Oman;
Mahad@du.edu.om
* Correspondence: author: c.algieri@itm.cnr.it (C.A.); sudip.chakraborty@unical.it (S.C.)
Abstract: Catalytic membrane reactors have been widely used in different production industries
around the world. Applying a catalytic membrane reactor (CMR) reduces waste generation from a
cleaner process perspective and reduces energy consumption in line with the process intensification
strategy. A CMR combines a chemical or biochemical reaction with a membrane separation process in
a single unit by improving the performance of the process in terms of conversion and selectivity. The
core of the CMR is the membrane which can be polymeric or inorganic depending on the operating
conditions of the catalytic process. Besides, the membrane can be inert or catalytically active. The
number of studies devoted to applying CMR with higher membrane area per unit volume in multi-
phase reactions remains very limited for both catalytic polymeric and inorganic membranes. The
various bio-based catalytic membrane system is also used in a different commercial application.
The opportunities and advantages offered by applying catalytic membrane reactors to multi-phase
systems need to be further explored. In this review, the preparation and the application of inorganic
membrane reactors in the different catalytic processes as water gas shift (WGS), Fisher Tropsch
synthesis (FTS), selective CO oxidation (CO SeLox), and so on, have been discussed.
Keywords: catalysis; membrane reactor; process intensification; inorganic catalyst; enzyme;
environmental applications
1. Inorganic Membrane Reactor
1.1. Introduction to Catalytic Inorganic Membrane Reactors
Since the conventional methodologies of chemical processes have been successfully
applied to synthesize enormous numbers of sophisticated products, researchers worldwide
have been searching for alternative methods, which are more efficient concerning energy
consumption, space reduction, and environmental safety [1]. One of the most promising
strategies to achieve these challenging goals is utilizing catalysts. Catalysts play an essential
role in numerous environmental transformations with high reaction regioselectivity and
stereospecificity. These peculiar characteristics allow scientists to apply them in modern
chemistry and organic synthesis processes. Anyway, the rapid growth of the chemical
industries for producing different chemicals requires improving manufacturing and pro-
cessing by reducing the equipment size, energy consumption, and waste production to
achieve sustainable and cheaper technologies (process intensification strategy) [1].
Membrane reactors, a process intensification technology, combine the membrane sepa-
ration process with chemical or biochemical reactions in a single unit [2]. This combination
determines higher conversion and improved selectivity and a compact and cost-effective
Catalysts 2021, 11, 691. https://doi.org/10.3390/catal11060691 https://www.mdpi.com/journal/catalysts