Journal of Research Updates in Polymer Science, 2014, 3, 149-156 149
E-ISSN: 1929-5995/14 © 2014 Lifescience Global
Characterization of Phosphate Glass Reinforced Gelatin Blend
Bioactive Composite Films
Kamol Dey
1,*
, Poonam Alamgir
2,3
, Shahnaz Parvin
2,3
, Gulshana Mohol
2,3
, Wafa Tonny
2
,
Mubarak A. Khan
2
and Ruhul A. Khan
2
1
Department of Applied & Environmental Chemistry, Faculty of Science, University of Chittagong, Chittagong-
4331, Bangladesh
2
Institute of Radiation and Polymer Technology, Bangladesh Atomic Energy Commission, Savar, Dhaka
1000, Bangladesh
3
Department of Chemistry, Jahangirnagar University, Savar, Dhaka, Bangladesh
Abstract: Bioactive composite films were prepared using bioresorbable phosphate glass powder and biodegradable
polymer gelatin (G) through solution casting process. Biocompatible monomer, 2-hydroxyethyl methacrylate (HEMA) was
used as the cross-linking agent and bioresorbable phosphate glass (PG) powder was used as reinforcement filler. The
composite films were obtained at various ratios of G, PG and HEMA. The PG modified gelatin composite (PG/G) film
was fabricated at a weight ratio of 12:88 while HEMA modified gelatin composite (HEMA/G) film at 50:50 ratio. On the
other hand, hybrid gelatin composite film, containing both PG and HEMA, was obtained using a G/PG/HEMA ratio of
44:12:44. Incorporation of PG improved the mechanical properties of the composite films. Morphological property of the
composite films was investigated by stereo microscope and it revealed that the composite films were porous in nature.
The thermal behaviour of the films was studied using thermogravimetric analysis. Water uptake of the films was also
performed.
Keywords: Gelatin, phosphate glass, bioactive, composite films, stereo microscope.
1. INTRODUCTION
Bioresorbable composite has gained tremendous
interest in the field of biomaterial research. Tissue
engineering has brought new challenges in this field in
terms of biodegradability, biocompatibility, homo-
geneity, osteoconductivity, vascularity, cell proliferation,
controlled release, mechanical properties [1-3]. Both
natural and synthetic polymers along with polylactic
acid, polyglycolide, polycaprolactone and their
copolymers, hydroxyapatite, calcium phosphate,
hyaluronate and hyaluronate derivatives have been
thoroughly studied to find a novel class of potential
application in tissue engineering [4-6]. Polymer
blending technique is simple and efficient to improve
the properties of polymer up to a desired level and has
been widely utilized in polymer modification field. It
offers reduced processing cost and versatility in the
selection of materials [7]. Polymer blending of
compatible materials leads to substantial enhancement
of mechanical and thermal performance [8-10]. A range
of materials with different properties can be
successfully blended to obtain fine tunable material for
a particular application [11]. Various nano-reinforc-
ement fillers such as silicate clay, carbon nanotubes,
*Address correspondence to this author at the Department of Applied &
Environmental Chemistry, Faculty of Science, University of Chittagong,
Chittagong-4331, Bangladesh; Tel: +88-031-2606001-10, 716552;
Fax: +88-031-2606014; E-mail: kamolacct@gmail.com, kamoldey@cu.ac.bd
graphene, calcium carbonate and phosphate glass are
being extensively studied in the field of nanocom-
posites. These nano fillers are capable of enhancing
the mechanical and thermal performance of the
polymer [12]. Our present research aims at developing
a biopolymer-organic-inorganic blend composite film
with enhanced mechanical and thermal properties. In
the present work, we chose phosphate based glass
(20Na
2
O-24CaO-16MgO-40P
2
O
5
) as a reinforcement
filler because of its some important criteria regarding
biomedical applications [13, 14]. The dissolution rate of
the glass can be altered varying the composition to
tailor the biomedical properties. The P
2
O
5
provides the
backbone structure of phosphate glass and has been
evolved as a promising biomaterial [15, 16]. The
organic phase of hard tissues contains type I collagen
[17, 18]. Gelatin is a denatured collagen and posse-
sses a wide range of biomedical properties making
suitable for tissue engineering [19, 20]. In the present
study, HEMA is used as a hydrophilic biocompatible
monomer. HEMA is a hydrophilic monomer and is
using in biomedical field [21]. Poly(HEMA) has also
adequate biocompatibility and uses in medical science
as implant [22]. The goal of this research work is to
determine the influence of PG and HEMA on the
preparation of a bio-artificial polymeric material using
gelatin polymer that would be used as an excellent
alternative to tissue scaffold material for artificial bone
tissue engineering and drug delivery.