1
A highly pH-sensitive Zn(II) chemosensor
Carla Bazzicalupi, Andrea Bencini, Silvia Biagini, Enrico Faggi, Giovanna Farruggia, Giulia
Andreani, Paola Gratteri, Luca Prodi, Alessio Spepi, Barbara Valtancoli
Electronic Supporting Information
Page2____________________ Experimental details for H
2
L
Page 3. Figure S1__________ Absorption spectra of 2’,7’-dichlorofluorescein in aqueous
solution at different pH values
Page 3. Figure S2__________ Fluorescence emission spectra of 2’,7’-dichlorofluorescein in
aqueous solution at different pH values
Page 4. Figure S3__________ Minimized conformations of [CdL(H
2
O)] complex.
Page 5. Figure S4__________ pH dependence of the absorbance at 505 nm (Cd(II), Pb(II)) or
498 nm (Cu(II)) as a function of pH compared to the distribution
curves of the complexes for a system containing H
2
L and Cd(II)
(a) Pb(II) (b) or Cu(II) (c) in 1:1 molar ratio
Page 6. Figure S5__________ ESI mass spectra recorded on a aqueous solution containing H
2
L
and Zn(II) in 1:1 (a) and 1:2 (b) molar ratios.
Page 7. Figure S6__________ Fluorescence emission intensity at 525 nm as a function of pH
compared to the distribution curves of the Cu(II) (a) or Pb(II) (b)
complexes for systems containing H
2
L and Cu(II) or Pb(II) in 1:1
molar ratio
Page 8. Figure S7__________ Flow cytometric evaluation of the intracellular fluorescence
distribution in unstained HL60 cells, H
2
L incubated cells and
H
2
L incubated, digitonin permeabilized cells.
Supplementary Material (ESI) for Dalton Transactions
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