Food Chemistry 46 (1993) 121-127
Low molecular weight coloured compounds
formed in xylose--lysine model systems#
Jennifer M. Ames, Anton Apriyantono
Department of Food Science and Technology, University of Reading, Whiteknights, Reading RG6 2AP, UK
&
Anna Arnoldi
Dipartimento di Scienze Molecolari AgroalimentarL Universitd degli Studi di Milano, Via Celoria 2, 1-2013.? Milano, Italy
(Received 28 January 1992; accepted 1 April 1992)
Aqueous solutions of xylose (1 M) and lysine monohydrochloride (1 M), initial
pH 5.27, were refluxed for 1 h, either by control of the pH at 5 (by the addition
of sodium hydroxide solution during heating) or without pH control (final pH
2.83). The ethyl acetate-extractable components were separated from each
model system and represented 0.41 and 0.36 + 0.05% (m/m), respectively, of the
initial reactants for the systems heated with and without pH control. Analysis
of the ethyl acetate-extractable components by TLC and HPLC (with diode
array detection) showed some similarities, but also many differencesbetween the
two systems. Two and seven coloured peaks were analysed, respectively, in the
systems heated with and without pH control, but only one was detected in both
systems. A novel coloured Maillard reaction product (detected only in the
model system heated without pH control) was isolated and purified by repeated
semi-preparative TLC and HPLC, prior to analysis by electronic absorption and
NMR spectroscopy and by low and high resolution FAB MS.
INTRODUCTION
The development of colour is the most obvious effect
of the Maillard reaction, but very little is known about
the chemical nature of the coloured compounds formed
(Nursten, 1986). Coloured Maillard reaction products
may be divided into two classes: the melanoidins,
which are brown and possess molecular weights of
several thousand daltons, and the low molecular weight
structures which typically comprise 2-4 linked rings
(Ames & Nursten, 1989).
Much of the information available on the low
molecular weight coloured Maillard reaction products
is the result of studies carried out by Ledl and his
co-workers in Munich and Stuttgart (Ledl, 1990; Ledl
& Schleicher, 1990). However, several of Ledl's studies
have been carried out in methanol or ethanol, rather
than in aqueous solution, or using amines rather than
amino acids. In fact, very few studies have reported
structural data for non-volatile coloured compounds
t Paper presented at the Royal Society of Chemistry sym-
posium on 'Non-enzymic browning', December 1991.
Food Chemistry 0308-8146/92/$05.00 © 1992 Elsevier Science
Publishers Ltd, England. Printed in Great Britain
121
formed from aqueous sugar-amino acid mixtures and
the structures of only five such compounds have been
elucidated worldwide (see Table 1) (Severin & Kronig,
1972; Ledl & Severin, 1978; Nursten & O'Reilly, 1983,
1986; Banks et al., 1988). An additional 29 compounds
were isolated from an aqueous xylose-glycine model
system and analysed by mass spectrometry only
(O'Reilly, 1982). They possessed relative molecular
masses in the region 149-448 D, and a furfuryl group
was evident in several of them. No doubt, the lack of
structural information available for coloured com-
pounds formed in sugar-amino acid model systems
is due to the highly complex mixtures of reaction
products obtained, and the consequent problems
encountered in isolating individual components in
adequate amounts for analysis by IR, NMR and mass
spectrometry.
The Maillard reaction is known to be greatly influ-
enced by the pH of the medium but, again, very little
information is available regarding the nature of the
coloured compounds formed in model systems heated
at different pH values. A comparison of the volatile re-
action products formed in a xylose-lysine model system
heated either with the pH controlled at 5 or without
pH control (final pH 2.83) revealed the formation of