Jointly published by React.Kinet.Catal.Lett.
Akadémiai Kiadó, Budapest Vol. 79, No. 1, 35-42
and Kluwer Academic Publishers, Dordrecht (2003)
0133-1736/2003/US$ 20.00.
© Akadémiai Kiadó, Budapest.
All rights reserved.
RKCL4147
MOLYBDENUM HDS CATALYSTS SUPPORTED ON NIOBIA-SILICA
Sonia Damyanova
a
*, Stanislava Andonova
a
, Iskra Stereva
a
, Chavdar
Vladov
a
, Lachezar Petrov
a
and Paul Grange
b
a
Institute of Catalysis, Bulgarian Academy of Sciences, 1113 Sofia, Bulgaria,
e-mail: soniad@satline.net
b
Université Catholique de Louvain, Unité de Catalyse et Chimie de Matériaux
Divisés, Place Croix du Sud, 2/17, 1348 Louvain-la-Neuve, Belgium
Received June 14, 2002
In revised form October 11, 2002
Accepted October 30, 2002
Abstract
The effect of the amount of Nb
2
O
5
on the dispersion and reductive properties of
Mo/Nb
2
O
5
-SiO
2
catalysts has been studied. Addition of niobium leads to an
increase of dispersion and the reducibility of molybdenum. A synergetic effect of
niobium on the catalytic activity in hydrodesulfurization of thiophene was
observed at 5.4 wt.% of Nb
2
O
5
.
Keywords: Niobia, molybdenum catalysts, hydrodesulfurization
INTRODUCTION
The present environmental problems open up a challenge for the
development of new hydrotreating catalysts, capable of decreasing the content
of heteroatoms in different oil cuts. The bifunctional catalysts for
hydrodesulfurization (HDS) are based on supported metal sulfides (MoS
2
or
WS
2
) and promoters (Co or Ni). The most commonly used support for these
catalysts is alumina [1,2], titania [3] or mixed oxides [4,5]. It is well known that
silica-supported molybdenum catalysts give lower HDS activity due to the
agglomeration of molybdenum species on the surface of silica caused by the
inertness of the support. Higher hydrotreating performances for these catalysts
can be achieved by changing the support composition, by addition of other
oxides that will lead to a modification of the textural properties as well as the
acid-base character of the support.