C. MI~ZII~RE, M. SALLI~ AND M. FOURMIGUI~ 2007
Data collection
Enraf-Nonius CAD-4
diffractometer
w/20 scans
Absorption correction: none
4100 measured reflections
3163 independent reflections
1754 reflections with
I > 2cr(/)
R,ot = 0.042
0m~., = 25.97 °
h = -1 ~ 11
k= -1 ---~ 16
1=-16---, 16
3 standard reflections
frequency: 60 rain
intensity decay: none
Sail& M., Gorgues, A., Jubault, M., Boubekeur, K.. Batail, P. &
Carlier, R. (1996). Bull. Soc. Chim. Fr. 133, 417-426.
Sall6, M., Jubault, M., Gorgues, M., Boubekeur, K., Fourmigu6, M.,
Batail, P. & Canadell, E. (1993). Chem. Mater. 5, 1196-1198
Sheldrick, G. M. (1990). Acta Crvst. A46, 467-473.
Shcldrick, G. M. (1993). SHELXL93. Program for the Refinement of
Crystal Structures. University of Gottingen, Germany.
Refinement
Refinement on F 2
R(F) = 0.040
wR(F2) = 0.086
S = 1.116
3163 reflections
199 parameters
H atoms constrained
w= 1/[cr~-(F,~) + (0.0448Pf
+ 0.5754P]
where P = (F,~ + 2F,2)13
(A/cr)m,~ < 0.001
Apmax = 0.480 e A,-3
Apmin = -0.365 e ~-3
Extinction correction: none
Scattering factors from
International Tables for
Crystallography (Vol. C)
Table 1. Selected bond lengths (A)
sI--cl 1.755 (4) $6--c13 1.737 (5)
sI--C3 1.776 (5) s6----c 12 1.756 f51
$2--c2 1.726 (5) $7---c9 1.740 (51
$2--C3 1.767 (4) S7~C8 1.854 (4)
$3~4 1.757 (41 $8~CI0 1.744 (5)
$3---C5 1.818 (51 S8---C8 1.839 (4)
$4~C4 1.760 (4/ C1--C2 1.347 (6)
$4---C6 1.810 (5) CI--CI 1 1.439 (6)
$5~C14 1.730 ~5) C3--C4 1.326 (6)
$5---C 12 1.761 (41
Data collection: CAD-4-PC (Enraf-Nonius, 1994). Cell refine-
ment: CAD-4-PC. Data reduction: XCAD4 (Harms, 1993). Pro-
gram(s) used to solve structure: SHELXS86 (Sheldrick, 1990).
Program(s) used to refine structure: SHELXL93 (Sheldrick,
1993). Molecular graphics: ORTEPII (Johnson, 1976). Soft-
ware used to prepare material for publication: SHELXL93.
Supplementary data for this paper are available from the IUCr
electronic archives (Reference: FG1493). Services for accessing these
data are described at the back of the journal.
References
Benahmed-Gasmi, A. S., Fr~re, P., Belyasmine, A., Malik, K. M. A..
Hursthouse, M. B.. Moore, A. J., Bryce, M. R.. Jubault. M. &
Gorgucs, A. (1993). Tetrahedron Len. 34. 2131-2134.
Cooper, W. F., Kenney, N. C., Edmonds, J. C., Nagel, A., Wudl, F.
& Coppens, P. (1971). J. Chem. Soc. Chem. Commun, pp. 889-890
Enraf-Nonius (1994). CAD-4-PC. Version 1.2. Enraf-Nonius, Delft.
The Netherlands.
Favard, J. F., Fr~re, P., Riou. A., Benahmed-Gasmi, A. S.,
Gorgues, A., Jubault, M. & Roncali, J. (1998). J. Mater. Chem.
8, 363-366.
Fr~re, P., Gorgues, A., Jubault, M., Riou, A., Gouriou, Y. & Roncali, J.
(1994). Tetrahedron Len. 35, 1991-1994.
Harms, K. (1993). XCAD4. Program for the Reduction of Enraf-
Nonius CAD-4 Diffractometer Data. University of Marburg, Ger-
many.
Johnson, C. K. (1976). ORTEPII. Report ORNL-5138. Oak Ridge
National Laboratory. Tennessee, USA.
Krebs, F. C., Larsen. J.. Boubekeur. K. & Fourmigu6, M. (1993). Acta
Chem. Stand. 47. 910-915.
Acta Cryst. (1998). C54, 2007-2009
Dibromo[(Z)-2-bromo-2-(hydroxymethyl)-
vinyl](n-butyl)tellurium(IV)
J. ZUKERMAN-SCHPECTOR, a* HI~LIO A. STEFANI, b
DIOGO DE 0 . SILVA, b ANTONIO L. BRAGA, c
LUCIANO DORNELLES, c CLAUDIO DA C. SILVEIRA c
AND I. CARACELLI d
~Laborat6rio de Cristalografia, Estereodin6mica e Mode-
lagem Molecular, Departamento Qu[mica, Universidade
Federal de S~o Carlos, Caixa Postal 676, 13565-905 S6o
Carlos, SP, Brazil, and lnstituto de Quimica-USP-SP, Brazil,
hFaculdade de CiEncias Farmacduticas, USP, Sdo Paulo, SP,
Brazil, 'Departamento de Qufmica, Universidade Federal de
Santa Maria, Santa Maria, RS, Brazil, and aDepartamento
F[sica, Universidade Federal de Sdo Carlos, SP, Brazil.
E-mail: julio@power, ufscar.br
(Received 17April 1998: accepted 14 July 1998)
Abstract
In the title compound, [TeBr2(C4H9)(C3H4BrO)] or
C7HI3Br3OTe, the primary geometry about the Te TM
atom is a pseudo-trigonal-bipyramidal arrangement
with axial bromines and one equatorial position
vacant. If an intermolecular secondary Te...O bond
of 3.041 (5)A, trans to the Te---C(vinylic) bond, is
taken into consideration, the structure may be re-
garded as pseudo-octahedral. Distances and angles are:
Te--Br 2.7295(10) and 2.6115(10), Te---C 2.092(6)
and 2.134 (7) ~,, Br--Te--Br 176.59(3), Br--Te--C
88.87(19), 89.0(3), 89.65(19) and 88.2(3), and C--
Te--C 99.7 (3) °. The lattice is formed by hydrogen-
bonded centrosymmetric dimers [O...Br = 3.399 (6)A],
which, in turn, are linked by the intermolecular sec-
ondary Te.-.O bond.
Comment
Vinylic tellurides are intermediates in the synthesis of
vinyllithium compounds, which are, in turn, important
intermediates in organic synthesis, either as precursors
of the widely used vinylcuprate compounds or as
nucleophiles leading to chain-elongation products by
© 1998 International Union of Crystallography
Printed in Great Britain - all rights reserved
Acta Cr3"stallographica Section C
ISSN 0108-2701 ©1998