Pharmacology & Pharmacy, 2010, 1, 69-74
doi:10.4236/pp.2010.12010 Published Online October 2010 (http://www.SciRP.org/journal/pp)
Copyright © 2010 SciRes. PP
69
The Study of Influence of Silica and Polyethilene
Glycols Organic-Inorganic Compounds on
Free-Radical Processes in Vitro
Olga G. Sitnikova
1
, Sergey B. Nazarov
1
, Irina V. Shikhanova
2
, Alexander V. Agafonov
2
,
Jean A. Dyuzhev
1
, Irina G. Popova
1
1
Ivanovo State Research Institute of Maternity and Childhood (RIMC), Ivanovo, Russia;
2
Institute of Solution Chemistry, Russian
Academy of Sciences, Ivanovo, Russia.
Email: ivgenlab@gmail.com
Received July 20
th
, 2010; revised August 10
th
, 2010; accepted September 30
th
, 2010.
ABSTRACT
In this study investigation of influence of hybrid nanosilica-polyethylene glycols materials (molecular weight 1500,
6000 and 15000), prepared by sol-gel synthesis, on lipid peroxidation and antioxidant activity of human serum in vitro
was performed. Methods included chemiluminescence analysis and quantitative malonic dialdehyde estimation. It was
revealed that nanosilica-PEG materials with different molecular weight had certain biological activity. Powders of
SiO
2
-PEG 1500 and SiO
2
-PEG 6000 manifest prooxidant effects, whereas mesoporous (calcine) powders produced
antioxidant effects in blood serum in vitro.
Keywords: Free-Radical Oxidation, Nanosilica, Chemiluminescence, Malonic Dialdehyde
1. Introduction
The study of free-radical processes of lipid oxidation and
antioxidant system is an important problem of modern
biomedicine. Oxygen is a powerful oxidant and oxy-
gen-mediated reactions are the main sources of energy
for variety of biological species. Metabolic processes
produce reactive oxygen species (ROSs), free radicals,
peroxides, malonic dialdehyde, Schiff's bases, which
damage membrane structures and lead to oxidative stress,
being the causative factor for a lot of widely spread dis-
eases, including reproductive disorders and prenatal inju-
ries [1-3].
Concerning this the role of antioxidants is to neutralize
toxic products of free-radical lipid peroxidation. In con-
ditions of excessive peroxidation the capacity of antioxi-
dant defense may decrease due to insufficient endogenic
antioxidant production or unfavorable environment fac-
tors [3]. Various substances are known to have antioxi-
dant activity; their investigation is of certain importance
for both biology and medicine [4].
Nowadays silica compounds attract considerable at-
tention. Silica stimulates fibroblastic activity of mesen-
chyma, promoting granulation and scarring. The lack of
silica may lead to depression of leukocyte activity in in-
flammation, poor wound scarring, anorexia, pruritus,
tissue flexibility decrease, skin turgor decrease, vascular
permeability increase and haemorrhagia as a result. Apart
from this silica antioxidant activity stands [5].
Investigators of peroxidation showed that silica pow-
ders stimulated active oxygen species and free radicals
production in culture of epithelial cells, resulting in cas-
pase activation and apoptosis [6]. Some authors experi-
mentally found out that inhalation of crystalloid silica in
animals lead to oxidative stress, inflammation and alveo-
lar fibrosis [7,8].
As a catalysts and functional composite materials spe-
cial attention is attracted by matrix hybrid silica derivates.
In this study we presented physical-chemical properties
of silica-based materials and their influence on peroxida-
tion processes in human serum. Silica nanoparticles are
biologically inert, have high adsorption rate, thermal and
mechanic stability, and therefore are expected to mani-
fest antioxidant activity.
The aim of the work was to study the influence of or-
ganic-innorganic silica and polyethylene glycols com-
pounds on free-radical processes in vitro.