ELSEVIER Thermochimica Acta 307 (1997) 97-106
thermochimica
acta
Effects of selected phenol derivatives on the autoxidation of linolenic
acid investigated by DSC non-isothermal methods
Grzegorz Litwinienko*, Teresa Kasprzycka-Guttman, Maciej Studzinski
Department of Chemistry, University of Warsaw, 02-093 Warsaw, Pasteura 1, Poland
Received 29 April 1997; received in revised form 25 August 1997; accepted 8 September 1997
Abstract
The kinetic features of the thermoxidation of linolenic acid (LNA) was investigated under non-isothermal conditions (50--
300°C) in the presence of the phenolic compounds: o-cresol, p-cresol, 2,4-dimethylphenol, 2,5-dimethylphenol, 3,5-
dimethylphenol, 2,4,6-trimethylphenol and 2,6-di-t-butyl-4-methylphenol at concentrations 0.26--20 mmol of compound per
mol of LNA. Temperatures of reaction onset at different heating rates were used to evaluate kinetic parameters of linolenic
acid thermoxidation by the Ozawa-Flynn-Wall method. Activation energy (Ea) of the pure linolenic acid thermoxidation was
70.4±0.5 kJ/mol and at the tested concentrations range of the phenolic compound, Ea increased maximally to 95.8±5.1 kJ/
mol for 2,6-di-t-butyl-4-methylphenol, 101.1±3.0kJ/mol for o-cresol, 90.9±l.5kJ/mol for 2,4,6-trimethylphenol,
89.9+4.4 kJ/mol (p-cresol), 80.7±4.5 kJ/mol (2,5-dimethylphenol) 86.1±3.6 kJ/mol (3,5-dimethylphenol) and 75.1-t-3.0 kJ/
mol for 2,4-dimethylphenol. At concentrations of the phenolic compound greater than 10 mmol per mol of LNA, a decrease of
inhibitory effect was observed. © 1997 Elsevier Science B.V.
Keywords: Activation energy; Antioxidants; DSC; Phenolic compounds; Linolenic acid
1. Introduction
Atmospheric oxygen is the most accessible and
economically important oxidising agent in many che-
mical processes in the petroleum and fat industries.
The production of large quantities of organic chemi-
cals, drying oils and modified polymers is based on the
controlled oxidation of hydrocarbons. However, auto-
xidation is an undesirable process since rubber, plas-
tics, fuel oil, fat and materials containing fat can
undergo autoxidative deterioration or rancidification
[1]. Unfavourable effects of oxidation are also
*Corresponding author. Fax: 0048 22 8225996; e-mail:
litwin @chem.uw.edu.pl
0040-6031/97/$17.00 © 1997 Elsevier Science B.V. All rights reserved
PII S0040-6031(97)00366-3
observed in biological systems, where pathological
events such as various diseases, cancer and ageing are
possibly caused by free radical oxidation of polyun-
saturated fatty acids, natural phospholipid membranes
and nucleic acids. The autoxidation of lipids and other
oxidizable substrates is a free-radical chain reaction
and after initiation (catalysed by light, transition metal
ions or water molecules), propagation of free hydro-
peroxy radicals occurs. This process can be repre-
sented by reaction:
ROO ° + RH + 02 -~ ROOH + ROO" (1)
An induction period is observed on the addition of
certain phenols [2], aminophenols [3] or carotenoids
[4], known as antioxidants, during the oxidation of