Electron-phonon interaction in disordered conductors: Static and vibrating scattering potentials
A. Sergeev and V. Mitin
Department of ECE, Wayne State University, Detroit, Michigan 48202
Received 2 July 1999; revised manuscript received 23 September 1999
Employing the Keldysh diagram technique, we calculate the electron-phonon energy relaxation rate in a
conductor with the vibrating and static -correlated random electron-scattering potentials. If the scattering
potential is completely dragged by phonons, this model yields the Schmid’s result for the inelastic electron-
scattering rate
e -ph
-1
. At low temperatures the effective interaction decreases due to disorder, and
e -ph
-1
T
4
l l
is the electron mean-free path. In the presense of the static potential, quantum interference of numerous
scattering processes drastically changes the effective electron-phonon interaction. In particular, at low tem-
peratures the interaction increases, and
e -ph
-1
T
2
/ l . Along with an enhancement of the interaction, which is
observed in disordered metallic films and semiconducting structures at low temperatures, the suggested model
allows us to explain the strong sensitivity of the electron relaxation rate to the microscopic quality of a
particular film.
I. INTRODUCTION
Electron-phonon scattering plays a key role in the descrip-
tion of many phenomena, such as electron dephasing, heat
removal from hot electrons, superconducting branch imbal-
ance relaxation, etc. Although well characterized in clean
bulk conductors, the current understanding in disordered and
nanoscale systems is limited.
Electron scattering from impurities and boundaries de-
stroys the single-particle picture of electron-phonon interac-
tion. Along with the process of ‘‘pure’’ electron-phonon
scattering, which takes place in pure conductors, there is the
other basic process, namely, the inelastic electron scattering
from vibrating impurities, defects, and boundaries. Together
with elastic electron scattering and pure electron-phonon
scattering, this mechanism generates a wide variety of inter-
ference processes. If the electron-scattering potential impu-
rities, defects, and boundaries is completely dragged by
phonons, the inelastic electron-impurity scattering may be
excluded by a unitary transformation to a frame of reference,
which moves with the phonon mode under consideration.
Exploiting this transformation, Schmid
1
has found that in the
presence of strong disorder ( q
T
l 1,q
T
is the wave vector of
a thermal phonon the electron-phonon interaction becomes
weaker, and the energy relaxation rate
e -ph
-1
is of the order of
( q
T
l )
0
-1
T
4
l (
0
-1
T
3
is the relaxation rate in pure mate-
rial. As emphasized in Refs. 2–4, this conclusion is consis-
tent with the Pippard’s famous result for the ultrasonic at-
tenuation coefficient. It was also demonstrated
2,5
that the
correct calculations lead to Schmid’s result and the Pippard
formula independent of the reference frame used.
Detailed studies show that many experimental results may
be understood in the frame of the available theory.
6–8
How-
ever, a set of low-temperature observations is in strong dis-
agreement with current theoretical understanding of the
electron-phonon interaction in disordered conductors. En-
hancement of the interaction due to disorder has been found
in two-dimensional electron gas 2DEG in GaAs/Al-Ga-As
heterojunctions with l =0.3-0.8 m below 0.5 K,
9
and in
bulk Ti
1 -x
Al
x
alloys with values of l ranged from 0.26 to 1.1
nm at T =3–10 K.
10
The T
2
dependence of the relaxation
rate is widely observed in experiments. In some cases it may
be associated with the contribution of transverse phonons in
the pure limit q
T
l 1, predicted by the theory. Recent
measurements
11
show that this dependence takes place even
in the deep impure limit q
T
l 0.01, where T
4
dependence is
expected.
As the current theory is self-consistent, the search for rea-
sons behind this discrepancy should turn to the model as-
sumptions. Many-body corrections to phonon states were
considered in Ref. 12. It has been found that the modification
of the electron relaxation rate occurs only under a strong
phonon damping. On the electronic side, the main model
assumption of the current theory is that the scattering poten-
tial is completely dragged by phonons. This assumption may
be wrong for structures with heavy defects and tough bound-
aries. That is why one can expect the relaxation rate to be
modified in nonhomogeneous conductors and nanoscale
structures.
To study the effects of incomplete drag of scatterers by
phonons we consider the model taking into account the vi-
brating and static -correlated random-scattering potentials.
One of the effects originating from elastic electron scattering
is well understood now. The diffusion motion of electrons
makes the interaction time longer, which enhances an inter-
action. Renormalization of the ‘‘pure’’ electron-phonon ver-
tex due to electron-impurity scattering has been calculated in
Ref. 13. Here we study all electron-phonon interference pro-
cesses, with taking into account the renormalization of all
vertices as well as the modification of electron screening due
to disorder.
The outline of this paper is as follows. Starting with bare
vertices of electron scattering from phonons, the static and
vibrating potentials, we consider screening of these vertices
and build effective vertices of the electron-phonon interac-
tion in Sec. II. The energy relaxation rate in a disordered
conductor is calculated in Sec. III. Discussion of our main
results and comparison with experiment are presented in Sec.
IV.
PHYSICAL REVIEW B 1 MARCH 2000-I VOLUME 61, NUMBER 9
PRB 61 0163-1829/2000/619/60417/$15.00 6041 ©2000 The American Physical Society