Supporting Information
Boronate-Modified Interdigitated Electrode Array for Selective
Impedance-Based Sensing of Glycated Hemoglobin
Yuwadee Boonyasit,
†,‡
Wanida Laiwattanapaisal,
§
Orawon Chailapakul,
#
Jenny Emnéus,
‡
and Arto R.
Heiskanen*
,‡,§
†
Graduate Program in Clinical Biochemistry and Molecular Medicine, Faculty of Allied Health Sciences, Chulalongkorn
University, Bangkok, 10330, Thailand.
‡
Department of Micro- and Nanotechnology, Technical University of Denmark, Kgs. Lyngby, 2800, Denmark.
§
Department of Clinical Chemistry, Faculty of Allied Health Sciences, Chulalongkorn University, Bangkok, 10330,
Thailand.
#
Electrochemistry and Optical Spectroscopy Research Unit (EOSRU), Department of Chemistry, Faculty of Science,
Chulalongkorn University, Bangkok, 10330, Thailand.
*E-mail: arto.heiskanen@nanotech.dtu.dk
Contents:
Figure S1 pH dependence of boronate-HbA1c interaction Page S-2
Figure S2 Optimization of glutaraldehyde and APBA concentration Page S-3
Figure S3 Optimization of immobilization (APBA) and incubation (HbA1c) time Page S-4
Figure S4 Sensing surfaces without boronate modification Page S-5
Figure S5 Precision profile (RSE% vs. HbA1c concentration) Page S-6
Figure S6 HbAo interference Page S-7
Figure S7 Regression plot for method bias (HbA1c % vs. HbA1c concentration) Page S-8
Table S1 Analytical characteristics of electrochemical boronate-based HbA1c sensors Page S-9
Table S2 Equivalent circuit parameters Page S-10
Table S3 Regeneration efficiency Page S-11