Eastern-European Journal of Enterprise Technologies ISSN 1729-3774 5/8 ( 113 ) 2021
66
Copyright © 2021, Authors. This is an open access article under the Creative Commons CC BY license
DEVELOPMENT
OF AN AMMONIA
PRODUCTION METHOD
FOR CARBON-FREE
ENERGY GENERATION
Sergey Zhadan
PhD, Engineer Researcher
Individual Entrepreneur «A.O. Dyba»
Kudryashova str., 7-B, Kyiv, Ukraine, 03035
Yevhenii Shapovalov
Corresponding author
PhD, Senior Researcher
Department of Knowledge Systems Creation
Junior Academy of Sciences of Ukraine
Degtyarivska str., 38/44, Kyiv, Ukraine, 04119
E-mail: sjb@man.gov.ua
Roman Tarasenko
Postgraduate Student
Institute of Telecommunications
and Global Information Space
Chokolivskyi blvd., 13, Kyiv, Ukraine, 03186
Anatoliy Salyuk
PhD, Professor
Department of Food Chemistry
National University of Food Technologies
Volodymyrska str., 68, Kyiv, Ukraine, 01601
Ammonia has great prospects in the context of the
transition to carbon-free energy. It can be used as fuel
in gas turbines, fuel cells, internal combustion engines,
and burned together with coal. However, industrial pro-
duction of ammonia is based on the Haber-Bosh process,
which involves the use of natural gas and coal, which, in
this case, does not make it really carbon-free. This study
proposes a method to produce ammonia, which is envi-
ronmentally friendly and does not require the use of fos-
sil fuels. It is based on the approach to adjusting the con-
centration of ammonium nitrogen in a biogas reactor and
implies the sorption of ammonia from the gas phase with
a solution of monoammonium phosphate, obtaining diam-
monium phosphate, and subsequently heating it with the
release of ammonia. The factors influencing the extraction
of ammonia from waste have been considered, as well as
the influence of temperature on the release of ammonia
from the solution of diammonium phosphate; the energy
efficiency of the method has been assessed. With increas-
ing temperature, the degree of ammonia and the degree of
sorbent regeneration increased. Under laboratory condi-
tions, 111 J/g of ammonia energy was spent. The higher
the concentration of (NH
4
)
2
HPO
4
in the solution, the less
energy is required to obtain a unit of ammonia mass. The
total amount of ammonia released varies depending on
the temperature. Sorbent regeneration can be carried out
using thermal energy obtained at a cogeneration plant.
The possibility of using this method to produce ammonia
at an industrial scale has been estimated by analyzing the
ways of ammonia utilization as a fuel. The potential for
ammonia production in the main livestock industries in
Europe and the United States is up to 11,482,651.15 and
11,582,169.5 tons per year, respectively. Applying this
solution also makes it possible to improve the efficiency of
biogas production from waste with high nitrogen content.
The proposed method of ammonia production could poten-
tially contribute to the development of carbon-free energy
Keywords: ammonia production, carbon-free ener-
gy, anaerobic digestion, ammonium nitrogen, ammonium
phosphates
UDC 662.767.2:636.5/.6
DOI: 10.15587/1729-4061.2021.243068
How to Cite: Zhadan, S., Shapovalov, Y., Tarasenko, R., Salyuk, A. (2021). Development of an ammonia production method for
carbon-free energy generation. Eastern-European Journal of Enterprise Technologies, 5 (8 (113)), 66–75. doi: https://doi.org/
10.15587/1729-4061.2021.243068
Received date 11.08.2021
Accepted date 17.10.2021
Published date 29.10.2021
1. Introduction
Much attention around the world is directed at reduc-
ing CO
2
emissions to prevent the negative effects of global
warming. The European Union has decided to reduce green-
house gas emissions by at least 55 % by 2030 compared to
1990 levels [1, 2]. In 2019, the European Commission an-
nounced plans to adjust the EU economic course to create
a climate and carbon-neutral space in Europe by 2050 [3, 4].
Most countries have set targets for future reductions
in greenhouse gas emissions. For example, the Japanese go-
vernment has identified national (INDC) contributions at
a 26.0 % reduction in greenhouse gas emissions by the fiscal
year 2030 compared to the fiscal year 2013 [5]. The Japanese
government has also set a long-term goal of reducing green-
house gas emissions by 80 % by the fiscal year of 2050 [6]. Ger-
many plans to reduce greenhouse gas emissions by 80–95 %
by 2050 [7]; the United Kingdom – by 80 % [8]; Japan,
France, and Canada – by 73–78 %; and Russia – by 48 % [9].
The UN estimates that cities account for up to 70 % of
global anthropogenic greenhouse gas emissions [10]. In this
regard, more than 100 cities announced their intention to be-
come carbon neutral by 2050. Some of them want to achieve
the goal earlier: Stockholm by 2040, Copenhagen by 2025,
and Liverpool by 2020 [8].
American Apple Inc. has announced a goal to reduce total
carbon dioxide emissions to zero across the entire supply and
production chain by 2030. Microsoft Corp. has announced
that it intends to achieve negative emissions by 2030, and,
by 2050, to completely eliminate the effects of carbon di-
oxide emissions over the entire time since the company was
founded in 1975 [11].
The reduction of CO
2
emissions into the atmosphere is
associated with the transition to carbon-free energy. This