Improvement of the Frequency Stability Below the Dick Limit With a Continuous Atomic Fountain Clock Laurent Devenoges, André Stefanov, Alain Joyet, Pierre Thomann, and Gianni Di Domenico Abstract—The frequency instability of a shot-noise limited atomic fountain clock is inversely proportional to its signal-to- noise ratio. Therefore, increasing the atomic flux is a direct way to improve the stability. Nevertheless, in pulsed operation, the local oscillator noise limits the performance via the Dick effect. We experimentally demonstrate here that a continuous atomic fountain allows one to overcome this limitation. In this work, we take advantage of two-laser optical pumping on a cold cesium beam to increase the useful fountain flux and, thus, to reduce the frequency instability below the Dick limit. A stabil- ity of 6 · 10 -14 τ -1/2 has been measured with the continuous cesium fountain FOCS-2. I. I S  the redefinition of the second in 1967, the stability and the accuracy of cesium atomic clocks have been continuously improved. With the advent of laser cooling in the early nineties, thermal beams were replaced by cold atomic fountains [1] to contribute to International Atomic Time (TAI) as primary frequency standards [2]. Currently, state-of-the-art pulsed fountain clocks (atoms are sequentially laser-cooled, launched ver- tically upwards, and interrogated during their ballistic flight before the cycle starts over again [3]) are operated at an accuracy level below 10 -15 in relative units. How- ever, their short-term stability is degraded by the phase noise of the interrogation oscillator via the Dick effect [4], [5]. For example, with a state-of-the-art boîtier à vieillissement amélioré (BVA; enclosure with improved aging) quartz oscillator, the excess noise resulting from the Dick effect limits the frequency stability of a pulsed fountain clock to approximately 10 -13 τ -1/2 [6]. This limit has been overcome in a few laboratories, either by using a cryogenic sapphire ultra-stable oscillator [7], or by gen- erating the microwave from an ultra-stable laser with the help of an optical frequency comb [8], [9]. Instead of making the effect negligible by employing an ultra-stable local oscillator, our alternative approach is to eliminate the dead times (time intervals without atoms in the free evolution region) by making use of a continuous beam of cold atoms. In this case, as shown in [10], the intermodulation effect 1 is negligible and the frequency sta- bility is only limited by the fountain signal-to-noise ratio. Therefore, increasing the atomic flux is a direct way to im- prove the short-term stability and reduce the integration time necessary to reach a given statistical resolution. In this work, we use two-laser optical pumping on a continu- ous beam of cold atoms to increase the useful fountain flux and thus to achieve a better stability. In Section II, we describe the continuous atomic foun- tain FOCS-2, its operation, and the state preparation with two-laser optical pumping. The experimental results will be presented in Section III and discussed in Section IV. Finally, we will conclude this work in Section V. II. D   C A F FOCS-2 A. Setup of the Fountain A scheme of the continuous atomic fountain FOCS- 2 is shown in Fig. 1 (a detailed description is given in [11]). Cesium atoms from a background thermal vapor are continuously slowed down in a two-dimensional magneto- optical trap (2D-MOT) to produce an intense beam of slow atoms (<25 m/s) [12]. This beam is then captured by a three-dimensional moving molasses which further cools and launches the atoms upward with a vertical velocity of 4 m/s [13]. This allows us to create a continuous beam of 10 9 atoms/s with a longitudinal temperature of about 75 μK [14]. The atomic beam is then collimated with Si- syphus cooling in the transverse directions to reduce the loss of flux resulting from thermal expansion during the free evolution time. Before entering the microwave cavity, the atoms are prepared into |F = 3, m = 0〉 with a state preparation scheme combining optical pumping and laser cooling. This is achieved in a 2-D-folded optical lattice situated 2.5 cm above the collimation stage. After these two steps, the transverse temperature is decreased to ap- proximately 3 μK. Finally, one last retro-reflected laser L. Devenoges, A. Joyet, P. Thomann, and G. Di Domenico are with the Laboratoire Temps-Fréquence, Université de Neuchâtel, Neuchâtel, Switzerland (e-mail: laurent.devenoges@unine.ch). A. Stefanov is with the Swiss Federal Office of Metrology, Bern-Wabern, Switzerland. 1 The intermodulation effect refers to the down-conversion of the local oscillator frequency noise into the bandpass of the frequency control loop by aliasing. The Dick effect is an example of the intermodulation effect characteristic of pulsed operation. 1