A Nanochannel Fabrication Technique
without Nanolithography
Choonsup Lee,* Eui-Hyeok (E. H.) Yang, Nosang V. Myung, and Thomas George
Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak GroVe DriVe,
Pasadena, California 91109
Received June 12, 2003; Revised Manuscript Received August 26, 2003
ABSTRACT
We have developed a new nanochannel fabrication technique using chemical-mechanical polishing (CMP) and thermal oxidation. With this
technique, it is possible to control the width, length, and depth of the nanochannels without the need for nanolithography. The use of sacrificial
SiO
2
layers allows the fabrication of centimeter-long nanochannels. In addition, the fabrication process is CMOS compatible. We have successfully
fabricated an array of extremely long and narrow nanochannels (i.e., 10 mm long, 25 nm wide, and 100 nm deep) with smooth inner surfaces.
Introduction. Nanofabrication of extremely small fluidic
structures provides powerful tools for the field of bionano-
technology.
1-4
Nanochannels are essential components in
nanofluidic systems. Among the many requirements for the
nanochannel fabrication technique are the following: It
should be cost-effective, able to precisely control channel
dimensions, and be CMOS compatible for ultimate integra-
tion with microelectronics. Previously, various nanochannel
fabrication techniques based either on e-beam lithography,
step sidewalls, or laser machining have been reported.
5-7
However, these techniques suffer from several limitations.
For example, e-beam lithography-based processes are rela-
tively expensive.
5
The step sidewall approach has limitations
in the maximum possible lengths of the nanochannel because
of lateral sacrificial etching effects.
6
Finally, laser machining
can only produce nanochannels with minimum widths in the
range of a few hundred nanometers and the fabrication
process is not CMOS compatible.
7
In this paper, we describe
the demonstration of a cost-effective nanochannel fabrication
technique with precisely controlled dimensions, using a
conventional CMOS fabrication process.
Experimental Section. Figure 1 shows the fabrication
procedures. First, 100 nm thick amorphous silicon is
deposited as shown in Figure 1a. The deposited amorphous
silicon thickness determines the depth of the nanochannel.
The photolithography is performed for determining the length
and shape of the nanochannel. And it is etched using reactive
ion etch (RIE) and subsequently oxidized in 1000 °C dry
O
2
for 40 min, as shown in Figure 1b. The SiO
2
thickness is
about 50 nm, which determines the width of the nanochannel.
Thus, the width of the nanochannel is controlled by adjusting
SiO
2
film thickness with the oxidation temperature or time.
8
The lower limit of the width in the nanochannel is about 5
nm, because the dry O
2
oxidation can readily produce 5 nm
SiO
2
film. And 500 nm thick amorphous silicon is deposited
as shown in Figure 1c. The overlayer thickness is ap-
proximately five times that of the amorphous silicon layer,
to minimize “dishing” effects. CMP process is performed
to expose the gap oxide as shown in Figure 1d. Then, the
gap oxide is vertically etched in the (10:1) buffered oxide
etch (BOE) for 20 min as shown in Figure 1e. The oxide in * Corresponding author. E-mail: choonsup.lee@jpL.nasa.gov.
Figure 1. Fabrication procedures. (a) SiN
x
and first amorphous Si
deposition; (b) RIE and dry O
2
oxidation for the nanometer gap;
(c) second amorphous Si deposition; (d) CMP until the gap oxide
is exposed. (e) The oxide in the nanometer gap is etched. (f) The
Au or oxide layer is used for sealing.
NANO
LETTERS
2003
Vol. 3, No. 10
1339-1340
10.1021/nl034399b CCC: $25.00 © 2003 American Chemical Society
Published on Web 09/16/2003