Eurasian J. Anal. Chem. 5(3): 227-238, 2010
Application of HPLC and HPTLC for the Simultaneous Determination of
Cefixime Trihydrate and Ambroxol Hydrochloride in Pharmaceutical
Dosage Form
Mahesh M. Deshpande
a
, Veena S. Kasture
b*
, Seema A.Gosavi
b
a
Department of Pharmaceutical chemistry, MGV’S College of Pharmacy, Panchvati, Nashik-03,
b
Sanjivani College of Pharmaceutical Education and Research, Kopargaon, Dist: Ahmednagar,
(M. S.), India, 423603.
Received: 13 August 2009; Accepted: 17 Februray 2010
Abstract
Two sensitive and reproducible methods are described for the quantitative determination for the
simultaneous estimation of cefixime trihydrate and ambroxol hydrochloride. The first method was
based on HPTLC followed by densitometric measurements of their spots at 254 nm. The separation
was on HPTLC aluminium sheets of silica gel 60 F254 using acetonitrile: methanol: triethylamine
(8.2:1:0.8, v/v/v) as mobile phase. The linear regression analysis was used for the regression line in the
range of 200 - 1000 ng spot
-1
for cefixime and ambroxol, respectively. This system was found to give
compact spots for cefixime and ambroxol, after development. The second method was based on HPLC
separation of the two drugs on the column [C18 (5 μ, 25 cm×4.6 mm, i.d.)] at ambient temperature
using a mobile phase consisting of acetonitrile: methanol (50:50, v/v). Quantitation was achieved with
UV detection at 254 nm based on peak area with linear calibration curves at concentration ranges 4 -
18 and 4 - 28 μg mL
-1
for cefixime and ambroxol, respectively. Both methods have been successively
applied to pharmaceutical formulation. No chromatographic interference from the tablet excipients
was found. Both methods were validated in terms of precision, robustness, recovery and limits of
detection and quantitation.
Keywords:
Cefixime; ambroxol; HPTLC; HPLC; method validation
1. Introduction
Cefixime (CFX) ((6R, 7R)-7-[(Z)-2-(2-amino-4-thiazolyl)-2-(carboxy-methoxyimino)
acetamido]-8-oxo-3-vinyl-5-thia-1-azabicyclo-[4,2,0]-oct-2-ene-2-carboxylic acid), is an
orally absorbed third generation cephalosporin antibiotic. It has a broad antibacterial spectrum
against various gram-positive bacteria and gram-negative bacteria, including Haemophilus
influenzae, Neisseria gonorrhoeae, Escherichia coli, and Klebsiella pneumoniae resistant to
ampicillin, cephalexin, cefaclor, and trimethoprim- sulfamethoxazole. Ambroxol, (AMB)
trans-4-(2-amino-3, 5-dibromobenzylamino) cyclohexanol hydrochloride is a compound with
potent mucolytic activity, for which it is used as an expectorant and bronchosecretolytic in
therapeutics [1-5]. The structures of drugs are shown in (Fig.1). Literature survey revealed
many chromatographic methods for determination of Cefixime alone or in combinations with
other drugs from pharmaceutical formulations and biological fluids [6-10]. Several
chromatographic methods have also been reported for determination of Ambroxol from
*
Corresponding Author
E-mail: veenakasture@hotmail.com
ISSN: 1306-3057, Moment Publication ©2010