toxins
Article
Antiparasitic Effects of Potentially Toxic Beetles (Tenebrionidae
and Meloidae) from Steppe Zones
Marta Díaz-Navarro
1,2
, Paula Bolívar
1,3
, María Fe Andrés
2
, María Teresa Gómez-Muñoz
3
,
Rafael A. Martínez-Díaz
4
,Félix Valcárcel
5
, Mario García-París
1
, Luis M. Bautista
1
and Azucena González-Coloma
2,
*
Citation: Díaz-Navarro, M.; Bolívar,
P.; Andrés, M.F.; Gómez-Muñoz, M.T.;
Martínez-Díaz, R.A.; Valcárcel, F.;
García-París, M.; Bautista, L.M.;
González-Coloma, A. Antiparasitic
Effects of Potentially Toxic Beetles
(Tenebrionidae and Meloidae) from
Steppe Zones. Toxins 2021, 13, 489.
https://doi.org/10.3390/toxins
13070489
Received: 16 June 2021
Accepted: 11 July 2021
Published: 14 July 2021
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1
Museo Nacional de Ciencias Naturales, CSIC, José Gutiérrez Abascal 2, 28006 Madrid, Spain;
maartadn@gmail.com (M.D.-N.); pbolivar@mncn.csic.es (P.B.); mparis@mncn.csic.es (M.G.-P.);
lm.bautista@csic.es (L.M.B.)
2
Instituto de Ciencias Agrarias, CSIC, Serrano 115-dpdo, 28006 Madrid, Spain; mafay@ica.csic
3
Facultad de Veterinaria, Universidad Complutense de Madrid (UCM), 28040 Madrid, Spain;
mariateresa.gomez.munoz@pdi.ucm.es
4
Facultad de Medicina, Universidad Autónoma de Madrid (UAM), Arzobispo Morcillo S/N,
28029 Madrid, Spain; rafael.martinez@uam.es
5
Grupo de Parasitología Animal, Departamento de Reproducción Animal, CSIC-INIA, 28040 Madrid, Spain;
valcarcel.felix@inia.es
* Correspondence: azu@ica.csic.es
Abstract: Arthropods and specifically beetles can synthesize and/or sequester metabolites from
dietary sources. In beetle families such as Tenebrionidae and Meloidae, a few studies have reported
species with toxic defensive substances and antiparasitic properties that are consumed by birds. Here
we have studied the antiparasitic activity of extracts from beetle species present in the habitat of
the Great Bustard (Otis tarda) against four pathogen models (Aspergillus niger, Meloidogyne javanica,
Hyalomma lusitanicum, and Trichomonas gallinae). The insect species extracted were Tentyria peiroleri,
Scaurus uncinus, Blaps lethifera (Tenebrionidae), and Mylabris quadripunctata (Meloidae). M. quadripunc-
tata exhibited potent activity against M. javanica and T. gallinae, while T. peiroleri exhibited moderate
antiprotozoal activity. The chemical composition of the insect extracts was studied by gas chro-
matography coupled with mass spectrometry (GC-MS) analysis. The most abundant compounds
in the four beetle extracts were hydrocarbons and fatty acids such as palmitic acid, myristic acid
and methyl linoleate, which are characteristic of insect cuticles. The presence of cantharidin (CTD)
in the M. quadripunctata meloid and ethyl oleate (EO) in T. peiroleri accounted for the bioactivity of
their extracts.
Keywords: Tenebrionidae; Meloidae; nematicide; antiprotozoal; GCMS; cantharidin; ethyl oleate;
otididae
Key Contribution: The antiparasitic activity of extracts from beetle species that may be present in
the diet of some birds support the hypothesis of their potential dietary antiparasitic effects.
1. Introduction
Arthropods contain secondary metabolites (defensins and toxins) characterized by
great chemical and biosynthetic diversity [1]. Specifically, coleopterans produce a wide
variety of active compounds or metabolites that are medicinal substances or precursors [2,3].
Other Coleoptera acquire toxic substances by sequestering secondary metabolites from
dietary sources, which are then transferred from invertebrates to upper trophic levels
within the ecosystem [1,4,5].
The consumption of secondary metabolites by animals can affect their parasite and
pathogen load, regardless of their toxicity to the animal itself. These effects are of particular
interest because there is an urgent need to search for natural products with therapeutic
Toxins 2021, 13, 489. https://doi.org/10.3390/toxins13070489 https://www.mdpi.com/journal/toxins