Nutrients 2021, 13, 3785. https://doi.org/10.3390/nu13113785 www.mdpi.com/journal/nutrients
Review
Margin of Exposure Analyses and Overall Toxic Effects of
Alcohol with Special Consideration of Carcinogenicity
Alex O. Okaru
1
and Dirk W. Lachenmeier
2,
*
1
Department of Pharmacy, University of Nairobi, Nairobi P.O. Box 19676-00202, Kenya;
alex.okaru@gmail.com
2
Chemisches und Veterinäruntersuchungsamt (CVUA) Karlsruhe, Weissenburger Straße 3,
76187 Karlsruhe, Germany
* Correspondence: lachenmeier@web.de; Tel.: +49-721-926-5434
Abstract: Quantitative assessments of the health risk of the constituents of alcoholic beverages
including ethanol are reported in the literature, generally with hepatotoxic effects considered as the
endpoint. Risk assessment studies on minor compounds such as mycotoxins, metals, and other
contaminants are also available on carcinogenicity as the endpoint. This review seeks to highlight
population cancer risks due to alcohol consumption using the margin of exposure methodology.
The individual and cumulative health risk contribution of each component in alcoholic beverages is
highlighted. Overall, the results obtained consistently show that the ethanol contributes the bulk of
harmful effects of alcoholic beverages, while all other compounds only contribute in a minor
fashion (less than 1% compared to ethanol). Our data provide compelling evidence that policy
should be focused on reducing total alcohol intake (recorded and unrecorded), while measures on
other compounds should be only secondary to this goal.
Keywords: alcohol; risk assessment; hepatotoxicity; dose–response relationship; margin of exposure;
epidemiological methods
1. Introduction
The epidemiological association of alcoholic beverages with cancer remains a topic
that has continued to attract global attention for over a century with the first documented
cases, cancer of the esophagus, being reported in 1910 [1,2]. Later in 1988, the World
Health Organization (WHO)/International Agency for Research on Cancer (IARC)
classified “alcohol drinking” as carcinogenic to humans (group 1) after establishing a
causal link between alcohol use and malignancies of the oral pharynx, esophagus, and
liver [1]. The promoters or causative factors in alcoholic beverages for developing
carcinogenic lesions are a matter of continuing debate among scientists. However,
alcohol being a multicomponent mixture, the potential contribution of each or all the
compounds to carcinogenesis should not be overlooked. These substances occur as
residues, contaminants, or even adulterants, in addition to being naturally occurring in
either raw materials or fermentation by-products.
Ethanol, the principal component of alcoholic beverages, is classified as a human
carcinogen (group 1) by IARC. Other than ethanol, other IARC-classified carcinogenic
compounds such as acetaldehyde, formaldehyde, acrylamide, aflatoxins, ochratoxin A,
arsenic, lead, cadmium, ethyl carbamate, furan, safrole, 4-methylimidazole,
N-nitrosodimethylamine (NDMA), 3-Monochloropropane-1,2-diol (3-MCPD), and
benzene have occurred in alcoholic beverages. The contribution of these compounds to
cancer is either synergistic or independent of each other. Understanding the contribution
of each component is important in disentangling the mechanisms of carcinogenicity due
to alcohol and ultimately aids in alcohol control policies. Nevertheless, epidemiological
Citation: Okaru, A.O.; Lachenmeier,
D.W. Margin of Exposure Analyses
and Overall Toxic Effects of Alcohol
with Special Consideration of
Carcinogenicity. Nutrients 2021, 13,
3785. https://doi.org/10.3390/
nu13113785
Academic Editor: Peter Anderson
Received: 29 July 2021
Accepted: 19 October 2021
Published: 25 October 2021
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