Food and Public Health 2016, 6(6): 157-164
DOI: 10.5923/j.fph.20160606.02
Supercritical Extraction of Cobia (Rachycentron canadum)
Liver Oil as a New Source of Squalene
Débora Nascimento e Santos, Eliane Hissae Takahashi,
Alessandra Barros Verde
,
Alessandra Lopes de Oliveira
*
Food Engineering Department, Faculty of Animal Science and Food Engineering, University of Sao Paulo, Pirassununga, Brazil
Abstract Cobia is a fish cultivated worldwide and there are few studies on the potential of their waste, such as the liver,
it's rich in oil and active compounds. The objective of this study was to extract cobia liver oil (CLO) using supercritical CO
2
under moderate temperature conditions (50, 60 and 70 °C, 250 bar) and characterize the oil (physico-chemical analysis, fatty
acids profile and squalene content). The results showed that CLO is rich in MUFA and presented squalene, suggesting that
this matrix can be applied in the production of high nutritional value oil.
Keywords Liver fish oil, Cobia, Supercritical extraction, Omega 3, Squalene
1. Introduction
Cobia, Canadum Rachycentron, is a marine fish native to
Brazil and found in tropical and subtropical seas. In captivity,
this fish presents a high growth rate with low incidence of
disease and produces high-quality meat [1, 2]. Because of
these attributes, this species has been widely used in
aquaculture in some countries in Asia and the Pacific region,
generating a product of great economic value [3]. In Brazil,
the production of cobia in captivity was initiated in 2006, and
it continues in expansion due to encouragement from the
Fishery Ministry and the private sector [4]. The cobia
growing in captivity generated stimulus for studies about
feeding and management techniques for growth efficiency.
The world production of fish, including fishing and fish
farming, was 158 million tons in 2012. Out of this total,
136.2 million tons (86% of total production) were used for
human consumption, and the remaining 14% (21.7 million
tons) was used for non-food purposes such as fishmeal and
fish oil production [5]. Fish oil extraction can be classified
into physical, chemical, and biological processes. The
chemical extraction, realised with organic solvents, is a
process well established. However, the use of toxic solvents
can result in protein denaturation and loss of functional
properties [6, 7]. In this context, supercritical fluid extraction
is a potential alternative for the many advantages that it
presents in relation to other methods.
Supercritical fluid extraction using CO
2
as a solvent can
be applied to obtain fish oil rich in unsaturated fatty acids at
* Corresponding author:
alelopes@usp.br (Alessandra Lopes de Oliveira)
Published online at http://journal.sapub.org/fph
Copyright © 2016 Scientific & Academic Publishing. All Rights Reserved
low temperatures. Supercritical CO
2
extraction produces no
oxygen in the process, which is responsible for the oxidation
of fatty acids. The supercritical CO
2
density can be easily
changed with temperature and pressure alteration, which
modifies the solvating power of the solvent. Another known
characteristic is the low toxicity of CO
2
that is recognised as
safe (GRAS) and still produces clean waste extraction and
solvent-free extracts [8, 9].
The first studies of the application of supercritical CO
2
extraction in fish oils were conducted in the 1950s. They
studied the phase equilibrium data and compounds of the fish
oils obtained by supercritical CO
2
and other organic solvents
[10]. Some studies have shown the fractions purification of
substances such as ethyl esters, eicosapentaenoic acid (EPA)
and docosahexaenoic acid (DHA) [11], acid esters of fish
oils [12], and contaminants [13]. In recent studies,
supercritical extraction has been applied for new fish species
or by-products [14] or as an extraction method combined
with other processes such as molecular distillation [15] in
order to optimise the fractionation of compounds with
biological activity such as alkylglycerols and squalene.
The objective of this research was to obtain cobia liver oil
(CLO) using supercritical extraction in different operational
conditions in order to characterise this oil by determining
physico-chemical parameters and the fatty acid profile and
by investigating the presence of bioactive compounds such
as squalene. In addition to the study of clean technology to
extract CLO, this study aimed to use waste from the fishing
industry, such as raw material, for the production of oil with
active properties.
2. Materials and Methods
2.1. Materials and Sample Characterisation