Hindawi Publishing Corporation
Advances in Meteorology
Volume 2010, Article ID 250896, 2 pages
doi:10.1155/2010/250896
Editorial
Marine Aerosol-Cloud-Climate Interaction
Nicholas Meskhidze,
1
Charles R. McClain,
2
Markus D. Petters,
1
Elisabetta Vignati,
3
Olaf Stetzer,
4
Chris Osburn,
1
and David J. Kieber
5
1
Department of Marine Earth and Atmospheric Sciences, North Carolina State University, Raleigh, NC, USA
2
NASA/Goddard Space Flight Center, Greenbelt, MD, USA
3
Joint Research Centre Institute for Environment and Sustainability Climate Change Unit, Ispra, VA, Italy
4
Institut f. Atmosph¨ are und Klima, Z¨ urich, Switzerland
5
Department of Chemistry, State University of New York, College of Environmental Science and Forestry, New York, USA
Correspondence should be addressed to Nicholas Meskhidze, nmeskhidze@ncsu.edu
Received 8 December 2010; Accepted 8 December 2010
Copyright © 2010 Nicholas Meskhidze et al. This is an open access article distributed under the Creative Commons Attribution
License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly
cited.
Concerns over the role of atmospheric aerosols in masking
observed climate change have sparked renewed interest in
the natural emissions of trace gases (functioning as aerosol
precursors) and aerosols. Understanding the aerosol budget
in the absence of anthropogenic influence is necessary to
establish a baseline aerosol forcing and provide a framework
for models to properly interpret the historical climate
record. Marine aerosol emissions, their composition, and
their effects on clouds and radiation budget remain poorly
characterized due to the large areal extent of the oceans
and resulting scarcity of observational data. It is therefore
not surprising that marine aerosols and associated cloud
processes play a major role and present a large uncertainty,
in predictions of future climate.
This special issue was motivated by our perceived need to
provide a platform for current discussions regarding marine
aerosol-cloud-climate interactions. Much research had been
performed in the 1950s–1970s following the discovery and
initial characterization of the bubble burst process by
Woodcock, Blanchard, McIntyre, Duce, and coworkers. A
special issue appeared in the Journal of Geophysical Research
in 1972 and research continued at a modest level over the
next decades. Renewed interest in the subject appeared in
the early 2000s, when a number of new studies identified
large fractions of organic material in ambient marine aerosol
in different locations, sparking an upsurge in laboratory,
field, satellite, and modeling studies. These studies aimed to
better characterize marine primary and secondary organic
aerosol production mechanisms, aerosol mass and number
fluxes, size-dependent sea spray enrichment factors, the split
between water soluble and insoluble organic fractions, the
chemical composition of organic aerosol, as well as to deter-
mine the effect of marine organics on cloud microphysical
properties. This special issue presents a snapshot of current
research topics in this study area. It comprises twelve peer-
reviewed open access articles spanning the full spectrum of
atmospheric science research on this subject.
A number of contributions address the chemical com-
position of marine aerosols. Rinaldi et al. present a reviews
and some innovative results on the chemical composition
of primary and secondary marine aerosol, showing sea-
sonal differences in nascent submicron sea spray particle
chemical composition collected at the Mace Head Atmo-
spheric Research Station. During low biological activity,
submicron marine aerosols were primarily composed of
sea salt, while particles collected during high biological
activity largely contained nonsea salt sulfate and organics.
Rinaldi et al. report distinct seasonal difference even in
the organic composition of submicron marine aerosol.
During low biological activity soluble and insoluble organic
compounds were comparable in abundance, while during
high biological activity submicron organics were dominated
by water soluble organic matter. Hawkins and Russell use
scanning Transmission X-ray Microscopy with Near-Edge
X-ray Absorption Fine Structure (STXM-NEXAFS) analysis
to classify marine primary organic aerosols collected in
the Arctic and southeastern Pacific marine boundary layers
into four major chemical types: carboxylic acid-containing