Evaluation of the Reactivity of Artificial Mixtures of Portland
Cement Clinker Obtained by Flame Spray Pyrolysis
ANDRÉS FELIPE PINTO, JORGE IVÁN TOBÓN, NATALIA
BETANCUR-GRANADOS and OSCAR JAIME RESTREPO-BAENA*
Cement and Construction Materials Group, Department of Materials and Minerals,
National University of Colombia Medellín Campus, Medellín 050036, Colombia.
Abstract
The Portland cement clinker consists of 95% calcium oxide, silicon,
aluminum and iron and 5% impurities of magnesium, sodium, potassium,
titanium, sulfur, phosphorus and manganese. The constituents of the
white clinker, formed from the combination of two or more of these main
oxides, correspond to alite (3CaO.SiO
2
or C
3
S), belite (2CaO.SiO
2
or
C
2
S) and celite (Ca
3
Al
2
O
6
or C
3
A), giving to cement its characteristic
properties. The fundamental properties of cement are its mechanical
resistance, chemical resistance, hydraulic behavior and heat release
during hydration. In this work, the reactivity of an artificial mixture of
white clinker, formed from alite, belite and celite prepared by flame
spray pyrolysis was evaluated. The phases were characterized by
X-ray diffraction, scanning electron microscopy and microcalorimetry, to
evaluate their formation and reactivity. The characterization showed that
during the synthesis of belite, a greater amount of the polymorph alpha
was produced, with some impurities. On the other hand, the synthesis
of celite allowed the production of the polymorph CII. The reactivity was
evaluated by microcalorimetry.
Material Science Research India
www.materialsciencejournal.org
ISSN: 0973-3469, Vol.16, No.(2) 2019, Pg.110-117
CONTACT Oscar Jaime Restrepo-Baena ojrestre@unal.edu.co Cement and Construction Materials Group, Department of
Materials and Minerals, National University of Colombia Medellín Campus, Medellín 050036, Colombia.
© 2019 The Author(s). Published by Oriental Scientific Publishing Company
This is an Open Access article licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International License
Doi:http://dx.doi.org/10.13005/msri/160204
Article History
Received: 30 March 2019
Accepted: 25 May 2019
Keywords
Flame Spray Pyrolysis,
Nanoparticles,
Reactivity,
Oxidant Flame,
Clinker.
Introduction
Portland cement is a type of material obtained from
the rotary kiln cooking of a mixture of limestone and
clay in a rotary kiln, which is brought to sinter to form
an intermediate product called clinker, which is mixed
with gypsum, giving rise to Portland cement.
1
The clinker consists of 95% of calcium oxides,
silicon, aluminum and iron and 5% of impurities
of magnesium, sodium, potassium, titanium,
sulfur, phosphorus and manganese. The main
constituents of the white clinker are correspond to
alite(3CaO.SiO
2
or C
3
S), belite (2CaO.SiO
2
or C
2
S)