Merit Research Journal of Medicine and Medical Sciences (ISSN: 2354-323X) Vol. 3(2) pp. 047-052, February, 2015
Available online http://www.meritresearchjournals.org/mms/index.htm
Copyright © 2015 Merit Research Journals
Original Research Article
Stability-indicating Colorimetric method for the analysis
of Niclosamide
*Shaza Wagiealla Shantier, Elrasheed Ahmed Gadkariem
and Mohamed Obeid Adam
Abstract
Department of Pharmaceutical
Chemistry, University of Khartoum
*Corresponding Author’s E-mail:
sshantier@yahoo.com
Tel: +249 9 12637509
Simple, accurate and stability-indicating colorimetric method was developed
for the determination of niclosamide in bulk and dosage forms. The method
was based on the alkaline hydrolysis of niclosamide with 0.1M sodium
hydroxide under the specified reaction conditions. The zero-order and first
derivative spectra of the degradation product (yellow colored) were
recorded at 380nm and 409nm respectively. Linearity was exhibited in the
concentration range 4-20μg/ml with good correlation coefficient (not less
than 0.999). The recovery percentage results (99.47 ± 1.30%, n=3) indicated
the absence of interference by the tablets recipients. The results obtained
by the developed method were statistically compared by the results of a
reported method for determination of niclosamide, and evaluated at 95%
confidence limits.
Keyword: Colorimetry, Degradation product, Derivative spectrophotometry,
Niclosamide, Zero-order
INTRODUCTION
Niclosamide (Figure 1) is orally administered
anthelmintics drug. It is highly effective against cestodes
infesting man-Taenia saginata, T.solium, Diphyllobo-
thrium latum and Hymenolepis nana, as well as
threadworm. It acts by inhibiting the oxidative
phosphorylation in mitochondria and interfering with
anaerobic generation of ATP by the tape-worm, as a
result tape-worm get partly digested in the
intestine (Tripathi, 2003; Rang and Dale, 2005; Goodman
and Gillman’s, 2001).
Recent reports claimed niclosamide as anticancer
agent. Niclosamide reported to inhibits the Wnt/βcatenin,
mTORC1, STAT3, NF-κB and Notch signaling pathways,
and induce cell cycle arrest, growth inhibition and
apoptosis (Li Y et al, 2014).
Various methods had been reported for the analysis of
niclosamide in bulk and dosage forms. These methods
include stability-indicating methods (Shaza et al., 2015),
chromatographic and spectrophotometric methods
(Daabees, 2000; Cholifah et al., 2008; Feyyaz and Nigar,
1994)
In the present work, a simple stability-
indicating colorimetric method was developed for the
determination of niclosamide in bulk and dosage
form.
Experimental/Instrumentation
UV spectrophotometric studies were carried out on
Shimadzu UV-1800ENG240V, (Koyoto, Japan).
MATERIALS
A drug sample of NA (Niclosamide tablets, 500mg) was
obtained from AlexiPharma, Egypt. The reference
standard, certified to contain 99%, was obtained from
Egypt. Sodium hydroxide (BDH), Pool, England;
Methanol Scharlau Chemie S.A., Spain; Acetone
Scharlau Chemie S.A., Spain.
Standard stock solution
NA standard solution (2.5 mg/ml) was freshly prepared i n
acetone. 1ml was further diluted with methanol to obtain