International Journal of Advancements in Research & Technology, Volume 3, Issue 11, November-2014
ISSN 2278-7763
Copyright © 2014 SciResPub.
Study of the Influence of Amorphous Tricalcium Phosphate on
Corrosion Inhibition of Mild Steel in Hydrochloric Acidic
Medium 1M
Hassan Elaidi
1
, Ilham Ismi
1
, Elhosseine Rifi
1
, Mouhsine Galai
2
, Rachid Touir
2
, Mohamed Ebn Touhami
2
, Zineb
Hatim
3
1
Laboratoire de synthèse organique et procédés d’extraction, Université Ibn Tofaïl, Faculté des Sciences , Kenitra, Maroc
2
Laboratoire d’Electrochimie de Corrosion et d’Environnement, Université Ibn Tofaïl, Faculté des Sciences , Kenitra, Maroc
3
Laboratoire d’Electrochimie et Traitement de Surface, Université chouaib doukkali, Faculté des sciences, El Jadida, Maroc
Email: hassanelaidi@yahoo.fr
ABSTRACT
In this study, the inhibition effect of amorphous tricalcium phosphate (TCPam) on mild steel corrosion in 1.0M HCl solution
was studied. For this aim, electrochemical techniques such as potentiodynamic polarization curves, weight loss (WL) and elec-
trochemical impedance spectroscopy (EIS) were used. It was shown that, the amorphous tricalcium phosphate (TCPam) acts as a
good inhibitor for mild steel corrosion in 1 M HCl solution. Its inhibition efficiency increased with concentration and reaches
87 % at 5×10
-6
M, and decreased with temperature and immersion time. Polarization measurements indicated that TCPam acts
as mexed type inhibitor. In addition, Mechanism of physical adsorption is proposed from the apparent activation energy (Ea).
Keywords : Amorphous Tricalcium Phosphate ;TCPam; Corrosion and Inhibition; Acidic medium, EIS
1 INTRODUCTION
RON and its alloys find utility in a wide spread spectrum of
many industrial units because of its low-cost and excellent
mechanical properties. For this reason, the corrosion behav-
ior of these materials has attracted the attention of several in-
vestigations. The mild steel has many industrial applications
because of its easy availability, uncomplicated fabrication of it
into water pipe lines [1- 2], cooling water systems [3], boilers
etc. However, they are susceptible to different forms of corro-
sion inducted by chloride and so on. Steel is the most corro-
sion vulnerable metal. Thus, much attention is given for its
protection from the hostile environments. Acid solutions are
widely used in industry. The most important areas of applica-
tion are acid pickling, industrial acid cleaning, acid descaling,
and oil-well acidizing[4–9]. HCl solution is one of the most
widely used agents for these goals. However, iron and its al-
loys could be corroded during these applications which result
in a waste of resources. Corrosion prevention systems favor
the use of chemicals with low or no environmental impacts.
The reduction in the corrosion rate of metals has numerous
advantages such as saving of resources, economic benefits
during the industrial applications, increasing the lifetime of
equipment and decreasing the dissolution of toxic metals from
the components into the environment. Therefore, inhibitors
are commonly used to minimize metal dissolution and acid
consumption. Various types of organic compounds are widely
used as corrosion inhibitors for protection materials against
corrosion deterioration [10]. A perusal of the literature on acid
corrosion inhibitors reveals that most organic substance em-
ployed as corrosion inhibitors act by adsorption on the metal
surface. Most of the efficient inhibitors used in industry are
organic compounds which mainly contain oxygen, sulphur,
nitrogen atoms and multiple bonds in the molecule through
which they are adsorbed on metal surface [11–19]. In recent
years, the méniral inhibitors have attracted more attention for
their excellent corrosion inhibition performance. These prod-
ucts dissociate in solution and it is their dissociation products
that ensure the phenomena of inhibition.
The aim of this study is to investigate the inhibition effect
of amorphous tricalcium phosphate (TCPam) on the mild
steel corrosion in 1.0 M HCl solution using weight loss and
electrochemical measurements.
2EXPERIMENTAL DETAILS
2.1 Materials
The steel used in this study is a mild steel (MS) with a
chemical composition (in wt%) of 0.21 % C, 0.38 % Si, 0.05%
Mn, 0.05 % S, 0.09 % P, 0.01 % Al and the remainder iron (Fe).
For weight loss tests, the rectangular coupons with the size of
3,7 cm × 1 cm × 0.2 cm were used. A columned mild steel
specimen, embedded in Teflon holder using epoxy resin with
an exposed area of 1 cm
2
, was used as the working electrode
for electrochemical measurements. The coupons and elec-
trodes were abraded with emery paper (up to 1200 grit),
cleaned with acetone and washed with distillated water, and
finally dried at hot air before being immersed in the acid solu-
tion. The aggressive solution (1 M HCl), used as blank, was
prepared by dilution of analytical grade 37%. The concentra-
tions of inhibitor were ranged from 10
-6
to 10
-4
M. The inhibitor
used was an amorphous tricalcium phosphate (Ca3 (PO4)2 n
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