VOL. 11, NO. 23, DECEMBER 2016 ISSN 1819-6608
ARPN Journal of Engineering and Applied Sciences
© 2006-2016 Asian Research Publishing Network (ARPN). All rights reserved.
www.arpnjournals.com
13681
SURFACE MORPHOLOGY AND INTERFACIAL BONDING BETWEEN
PALM FIBER TREATED WITH SEA WATER AND SAGO MATRIX
Mardin Husen, Muhammad Balfas, Kusno Kamil
Departement of Mechanical Engineering, Universitas Muslim Indonesia, Makassar, Indonesia
E-mail: mardin@umi.ac.id
ABSTRACT
Surface morphology, roughness and bonding among palm fibers and sago matrix were observed. The sugar palm fiber was
treated by sea water immersion with duration of 1, 2, 3 and 4 weeks, before naturally dried under the sun for 3 hours then
continued by 6 hours oven at 80°C. SEM, XRD and roughness arithmetic tests are applied to see the surface morphology,
roughness and bonding among fibers and the matrix. The result shows that fibers morphology and roughness changes with
immersion duration. At longer immersion duration the roughness increases and the fiber-matrix quality is better. The best
interlocking of matrix and fibers occurred after duration of 4 weeks fiber immersion, where no more gaps seen between the
fiber and matrix.
Keywords: palm fiber, submersion, surface morphology, sago matrix, bonding.
INTRODUCTION
Cellulose-based natural fibers become a challenge for
researchers to reveal their advantages compare to synthetic
fibers, including the application possibilities to the global
construction and engineering technology [1]. Natural palm
fibers (Arenga pinata) have the prospect to be developed
as reinforcement substance in composite material due to
its flexural properties, salt water resistance,
environmentally friendly and relatively high tensile
strength [2]. Most of natural fibers are hydrophilic in
nature, strongly opposite to the hydrophobic properties of
polymer. Hence, soaking natural fiber in ocean water is
intended to reduce the hydrophilic characteristic of natural
fibers and presume to be more hydrophobic compatible to
the polymer materials [2, 3].
Sea water immersion cleans the extractive media off
the natural fibers such as lignin, pectin, wax and dirt
(impurities) in order to obtain surface with relatively
uniform topography. Topography of fiber surface affected
by soaking treatment is reviewed qualitatively through
observation by Scanning Electron Microscopy [4]. While
quantitative characteristics of the fiber surface were
observed by direct measurement of Roughness Arithmetic
Surface Area, which provides information about porosity
and roughness [5]. Change on the surface shapes were
observed by comparing the differences of roughness
patterns between the immersed fibers (treatment) and the
untreated fibers (green fiber).
Fiber characteristics on morphology and surface
roughness are crucial information for composite
reinforcement applications [6]. With the increasing
awareness of environmental protection, natural fibers
should contribute to a cleaner environment while meet
today’s considerable demand of composites [7]. Natural
fibers such as flax, hemp and jute are some of the most
commonly used reinforcement material of fiber composite.
Composites of polymers-reinforced natural fibers should
be more eco-friendly as the reinforcement and matrix
material (eg. polylactide - PLA) are degradable, as this
bio-composites commonly named as "green composites"
[8-9].
Although environmentally friendly, natural fibers
have a major drawback associated with application for
reinforcement of polymer matrix, such as problems
associated with surface of natural fibers and polylactide.
Several approaches have been made to the surface
modification of cellulose (e.g. esterification of cellulose
and cellulose substrate to graft copolymerization) and the
use of multiple adjustments, i.e. maleated polylactide and
isocyanate [7-9]. Several studies have been done to give
more utilization of natural fibers focusing the issues of
adhesion among natural fibers and the polymer matrix
including opposite chemical properties of hydrophilic
natural fibers and hydrophobic polymer matrix. Other
factors include surface area, surface structures and
porosity of the fiber relatively neglected in consideration
of adhesion among surface fiber and the matrix [9].
The morphology and roughness of the surface of the
natural fiber has been recognized as a significant factor for
composite reinforcement. Its effects on the performance of
composites have been investigated by the interfacial shear
strength of fiber surface roughness through Scanning
Electron Microscope [10]. Characteristics of natural fiber
differenced from commercial synthetic fibers in terms of
geometry, morphology, and surface profiles. This study
observe the effects of sea water on fiber surface
morphology and roughness so that the interface of sugar
palm fiber of sago matrix may be improved to be
considered as bio-composite material. SEM and roughness
arithmetic are utilized to analyze the surface morphology
and roughness of the fiber surfaces.
Most of natural fibers consist of high cellulose with
difference in particular micro structure. These particular
microstructure have strong bonds of intra- and
intermolecular hydrogen which are various in sizes. The
larger the molecule size, the weaker the bond, and the
smaller the molecular size, the stronger their bonds.
Hence, microstructures affect the tensile strength of fibers.
As microstructures of palm sugar fiber consist of 85%
cellulose, and covering almost the whole fibers surface,
the fibril bonds then become stronger.