Metabolites 2021, 11, 755. https://doi.org/10.3390/metabo11110755 www.mdpi.com/journal/metabolites
Article
Glutamine Homeostasis and Its Role in the Adaptive Strategies
of the Blind Mole Rat, Spalax
Dmitry Miskevich
1,
*, Anastasia Chaban
1
, Maria Dronina
2
, Ifat Abramovich
3
, Eyal Gottlieb
3
and Imad Shams
1,2,
*
1
Department of Evolutionary and Environmental Biology, Faculty of Natural Sciences, University of Haifa,
Haifa 3498838, Israel; anastasia@chaban.su
2
Institute of Evolution, University of Haifa, Haifa 3498838, Israel; dronina.maria@gmail.com
3
Technion Faculty of Medicine, Haifa 3525433, Israel; ifat.a.g@gmail.com (I.A.); e.gottlieb@technion.ac.il (E.G.)
* Correspondence: miskevichd@gmail.com (D.M.); imad.shams@univ.haifa.ac.il (I.S.)
Abstract: Oxidative metabolism is fine-tuned machinery that combines two tightly coupled fluxes
of glucose and glutamine-derived carbons. Hypoxia interrupts the coordination between the me-
tabolism of these two nutrients and leads to a decrease of the system efficacy and may eventually
cause cell death. The subterranean blind mole rat, Spalax, is an underexplored, underground, hy-
poxia-tolerant mammalian group which spends its life under sharply fluctuating oxygen levels.
Primary Spalax cells are an exceptional model to study the metabolic strategies that have evolved in
mammals inhabiting low-oxygen niches. In this study we explored the metabolic frame of gluta-
mine (Gln) homeostasis in Spalax skin cells under normoxic and hypoxic conditions and their im-
pacts on the metabolism of rat cells. Targeted metabolomics employing liquid chromatography
and mass spectrometry (LC-MS) was used to track the fate of heavy glutamine carbons (
13
C5 Gln)
after 24 h under normoxia or hypoxia (1% O2). Our results indicated that large amounts of gluta-
mine-originated carbons were detected as proline (Pro) and hydroxyproline (HPro) in normoxic
Spalax cells with a further increase under hypoxia, suggesting a strategy for reduced Gln carbons
storage in proteins. The intensity of the flux and the presence of HPro suggests collagen as a can-
didate protein that is most abundant in animals, and as the primary source of HPro. An increased
conversion of αKG to 2 HG that was indicated in hypoxic Spalax cells prevents the degradation of
hypoxia-inducible factor 1α (HIF-1α) and, consequently, maintains cytosolic and mitochondrial
carbons fluxes that were uncoupled via inhibition of the pyruvate dehydrogenase complex. A
strong antioxidant defense in Spalax cells can be attributed, at least in part, to the massive usage of
glutamine-derived glutamate for glutathione (GSH) production. The present study uncovers addi-
tional strategies that have evolved in this unique mammal to support its hypoxia tolerance, and
probably contribute to its cancer resistance, longevity, and healthy aging.
Keywords: glutamine; metabolome; hypoxia; proline cycle; GSH; adaptation; bioenergetics
1. Introduction
Glucose (Glc) and glutamine (Gln) are two central metabolic nutrients that maintain
cellular metabolism. Gln has a more pleiotropic role in cellular metabolism than Glc. It
incorporates directly into proteins [1] and participates in the proteostasis regulation [2];
provides carbons and nitrogen for the biosynthesis of amino acids, nucleotides, and
hexosamines [1,3,4]; replenishes the tricarboxylic acid (TCA) cycle with carbons [5]; and
plays an important role in the gluconeogenesis (GNG) [6].
Hypoxia upregulates the level of hypoxia-inducible factor 1α (HIF-1α) which
switches cellular bioenergetics to anaerobic mode [7]. The anaerobic mode includes re-
duced pyruvate metabolism, uncoupling of the glycolysis and the TCA cycle, and the
subsequent shortage of glucose-derived acetyl-CoA (Ac-CoA) [8,9]. In turn, the deficit of
ac-CoA could result in a decreasing citrate (Citr) level that is essential for multiple bio-
Citation: Miskevich, D.; Chaban, A.;
Dronina, M.; Abramovich, I.;
Gottlieb, E.; Shams, I. Glutamine
Homeostasis and Its Role in the
Adaptive Strategies of the Blind
Mole Rat, Spalax. Metabolites 2021,
11, 755. https://doi.org/10.3390/
metabo11110755
Academic Editors: Matthew Pa-
menter and Ken Storey
Received: 9 October 2021
Accepted: 30 October 2021
Published: 31 October 2021
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