Journal of Applied Pharmaceutical Science Vol. 8(08), pp 012-020, August, 2018
Available online at http://www.japsonline.com
DOI: 10.7324/JAPS.2018.8802
ISSN 2231-3354
© 2018 Haryati Ahmad Hairi et al. This is an open access article distributed under the terms of the Creative Commons Attribution License -NonCommercial-
ShareAlikeUnported License (http://creativecommons.org/licenses/by-nc-sa/3.0/).
*
Corresponding Author
Ahmad Nazrun Shuid, Department of Pharmacology, Faculty of
Medicine, Pre clinical Building, Universiti Kebangsaan, Malaysia,
Jalan Yaacob Latiff, Bandar Tun Razak, Cheras, 56000 Kuala Lumpur.
E-mail: anazrun @ yahoo.com
Demethylbelamcandaquinone B Isolated from Labisia Pumila
Haryati Ahmad Hairi
1
, Jamia Azdina Jamal
2
, Nor Ashila Aladdin
2
, Khairana Husin
2
, Noor Suhaili Mohd Sof
1
,
Norazlina Mohamed
1
, Isa Naina Mohamed
1
, Ahmad Nazrun Shuid
1*
1
Department of Pharmacology, Faculty of Medicine, Preclinical Building, Universiti Kebangsaan Malaysia, Jalan Yaacob Latiff, Bandar Tun Razak, Cheras,
56000 Kuala Lumpur, Malaysia.
2
Faculty of Pharmacy, Universiti Kebangsaan Malaysia, Jalan Raja Abdul Aziz, 50300 Kuala Lumpur, Malaysia.
ARTICLE INFO ABSTRACT
Article history:
Received on: 19/05/2018
Accepted on: 19/07/2018
Available online: 31/08/2018
(LP) or more commonly known as Kacip Fatimah in Malaysia has received much attention due to its
estrogenic effects, including its role in the treatment of osteoporosis. This study was designed to explore the active
compound of LP that may be responsible for its anti-osteoporotic effects. Crude aqueous extract of
var alata (LPva) was fractionated into hexane (Hex), dichloromethane (DCM) and methanol (Met) solvents and
their proliferative effects on mouse osteoblastic cell line (MC3T3-E1) were evaluated with MTS bioassay. The DCM
fraction signifcantly promoted cell proliferation in a dose-dependent manner. Thin layer chromatography (TLC) was
performed on the DCM fraction of LPva to separate the constituents and the potential active compound was identifed.
Further isolation was achieved by column chromatography (CC) and Sephadex LH-20 column chromatography. The
bioactivity of the isolated compound was confrmed by its ability to replicate MC3T3-E1 accelerated proliferation
and differentiation. Mass spectrometry and nuclear magnetic resonance (NMR) identifed the active compound as
demethylbelamcandaquinone B. Further studies are required to determine the potential of this active compound of
LPva in treating osteoporosis.
Key words:
active compound, Labisia
pumila, osteoporosis,
osteoblasts.
INTRODUCTION
Osteoporosis, a worldwide prevalence of disease, can be
defned as a systemic skeletal disease characterized by weak bones
and high risk of fractures (Kanis and Johnell, 2006). This disease
generally affects the elderly population and is associated with
postmenopausal estrogen defciency and progressive bone loss
(McCann et al., 2008; Pisani et al., 2016). Low estrogen level leads
to excessive bone resorption and reduced bone formation (Bord
and Beavan, 2003; Sorensen et al., 2006). The imbalance of bone
remodeling resulted in a bone loss and eventually osteoporosis
(Feng and Mcdonald, 2011). The main option for prevention and
treatment of postmenopausal osteoporosis is hormone replacement
therapy (HRT). However, HRT was linked to breast carcinoma
(Kotsopoulos et al., 2016), endometrial cancer (Chlebowski
et al., 2016) and cardiovascular disease (Bassuk and Manson,
2016). Bisphosphonate is a synthetic drug used to reduce the risk
of vertebral and hip fractures, but daily bisphosphonate therapy
may cause esophagitis and osteonecrosis of the jaw (Xu et al.,
2013). Selective estrogen receptor modulator or SERM is another
synthetic drug that binds to the intracellular estrogen receptors in
target organs as agonists or antagonists. Unfortunately, it may also
cause serious side effects such as thromboembolic disorders and
hot fushes (Maximov et al., 2013).
Recently, phytoestrogen became a favorable alternative
therapeutic agent for treatment of osteoporosis. Phytoestrogens,
such as isofavones (Deyhima et al., 2003; Singh et al., 2015),
lignans (Zhu et al., 2017) and coumestans (Ueda et al., 2011) acted
as SERMs to exert therapeutic effects against postmenopausal
osteoporosis. These phytoestrogens could also promote calcium
absorption or regulate bone remodeling through estrogen receptor
Labisia pumila
Labisia pumila
Enhanced Proliferation and Differentiation of Osteoblast Cells
Labisia pumila