Research J. Pharm. and Tech. 13(8): August 2020
1
ISSN 0974-3618 (Print) www.rjptonline.org
0974-360X (Online)
RESEARCH ARTICLE
Development and Validated Stability indicating RP-HPLC method for
quantitative determination of Ascorbic acid and piperine in
Dhathryaristam
Dr Paramita Das, Dr Padmavathi. P. Prabhu, Jithender Reddy
1
Dept of Pharmaceutical Chemistry, Krupanidhi College of Pharmacy, Bengaluru, Karnataka
2
Srinivas College of Pharmacy, Mangalore, Karnataka
3
Vaageswari College of Pharmacy, Telangana
*Corresponding Author E-mail: paramitadas04@gmail.com
ABSTRACT:
Dhathryaristam is an ayurvedic medicine described in Charaka samhita chikitsasthana. The preparation consists
of Phyllanthus emblica (amlaki, Indian goose berry) and Piper longam (Indian long pepper). The aim of this
research was to determine a finger print methods for ascorbic acid and piperine using simple mobile
phase((buffer: acetonitrile) in raw material as well as formulation. The efficient separation of chemical marker
was carried out using reverse phase C18 eluted with gradient mobile phase. The separation occurred at 4.1min
ascorbic acid and 5.6min piperine. Method validation was demonstrated by system suitability, accuracy,
precision, repeatability and recovery. The calibration curve was found to be within the tested ranges. The
recoveries were between 98-102%. The photo degradation studies exhibit the formation of various degraded
product. The quantification of ascorbic acid in raw material was 1.917μg/ml in Phyllanthus emblica and
marketed formulation D-I and D-II are 1.877μg/ml and 1.871μg/ml respectively. The quantification of piperine
in raw material was found to be 10.106μg/ml in Piper longam in two marketed formulation D-I and D-II are
10.845 μg/ml and 10.106μg/ml respectively. The developed and validated method can be effectively applied to
the quantitative determination of herbal formulation containing ascorbic acid and piperine.
KEYWORDS: Dhathryaristam, Phyllanthus emblica, Piper longam, marker, Quantification.
INTRODUCTION:
Ayurveda is one of the world’s oldest holistic medicine
systems also known as “mother of all healing”. In India,
plant based products are commonly used while; poly-
herbals have existed worldwide with a long history and
are used in various ayurvedic therapies
1
. A key challenge
for scientist in developing a polyherbal formulation is to
develop a well-designed methodology and quantitative
analysis of marker for standardization of herbal
medicine. Quantitative estimation of chemical marker in
polyherbal formulation is always difficult task
2
.
Standardization of herbal drug is challenging in terms of
modern parameter.
Received on 25.04.2020 Modified on 11.06.2020
Accepted on 05.08.2020 © RJPT All right reserved
Research J. Pharm. and Tech. 2020; 13(8):.
DOI:
The specific guidelines for the same have set by WHO
for the evaluation of herbal drugs. Lot of advancement
has taken place in chromatographic techniques; mostly
RP-HPLC with gradient elution is most commonly used
for polyherbal formulations. Markers can be separated
by different separation techniques with good resolution
and less interference from each other. Dhathryaristam
also known as Amalakarishtam is an herbal medicine
consists of Phyllanthus emblica (ascorbic acid) and
Piper longam (piperine). Ascorbic acid{R-3,4-
dihydroxy-5-((S)-1,2-dihydroxyethyl) furan-2(5H)-
one}is hydro soluble compound and plays an essential
role in defence against radical oxygen species
3
. Piperine
{(2E,4E)-5-(2H-1,3-Benzodioxol-5-yl)-1-(piperidin-1-
yl) penta-2,4-dien-1-one} having potent bronchodilator
properties. Dhathryaristam contains 5-10% of self
generated alcohol. Ascorbic acid and piperine are
excellent herbs that have been considered for various
formulations. It has been proven that ascorbic acid
extract has strong antioxidant
4
properties and protect
against immune deficiencies
5
. Piperine has got