Biocidal Polystyrene Beads. III. Comparison of N-halamine
and Quat Functional Groups
Y. Chen,
1
S. D. Worley,
1
T. S. Huang,
2
J. Weese,
2
J. Kim,
3
C.-I. Wei,
4
J. F. Williams
5
1
Department of Chemistry, Auburn University, Auburn, Alabama 36849
2
Department of Nutrition and Food Science, Auburn University, Auburn, Alabama 36849
3
Korea Atomic Energy Research Institute, 150, Duckjin-dong, Yuseong-Gu, Daejeon, 305-353, Korea
4
Department of Nutritional Sciences, Oklahoma State University, Stillwater, Oklahoma 74078
5
Vanson-HaloSource Corporation, Redmond, Washington 98052
Received 21 August 2003; accepted 8 November 2003
ABSTRACT: A comparison has been made between the
biocidal efficacies of N-chlorinated polymeric beads and two
derivatives of polyquat beads. Biocidal effects were mea-
sured after brief contact exposures of aqueous suspensions
of either Staphylococcus aureus or Escherichia coli to the water-
insoluble beads. The polymeric backbone was held the same
in all three types of beads, so they differed only in their
biocidal derivative moieties. In all cases, functionalization of
crosslinked chloromethylated polystyrene beads was per-
formed to introduce the biocidal properties. Synthetic meth-
ods and test data will be presented. The most effective
biocide, as measured by degree of inactivation in the short-
est contact time of the two species of bacteria, was the
N-chlorinated hydantoinyl derivative of methylated poly-
styrene. © 2004 Wiley Periodicals, Inc. J Appl Polym Sci 92:
363–367, 2004
Key words: biocidal polymers; N-halamine polymers; poly-
quats
INTRODUCTION
The most widely employed biocidal materials in use
today in disinfecting household products are quater-
nary ammonium salt derivatives (quats) and their
polymeric derivatives (polyquats). It is thought that
the mechanism of action of quats and polyquats
against pathogenic microorganisms involves first the
adsorption of the positively charged site of the mole-
cule onto the cell wall. This is then followed by diffu-
sion through the cell wall to bind with and disrupt the
cytoplasmic membrane, and then release of alkyl cat-
ions and constituents of the cytoplasmic membrane,
causing death of the cell.
1
These materials have several
advantages which have escalated their use and popu-
larity in society. They are generally stable in aqueous
solution for extended periods and have long shelf
lives. If properly designed with structures containing
satisfactory lipophilic alkyl groups, such as dodecyl,
they can be effective against a broad spectrum of
pathogenic microorganisms. Most important, many of
them have received approval by the government-reg-
ulatory agencies for commercial sales. However, they
also have limitations. Contact times for disinfection tend
to be lengthy, and they cannot be regenerated once lost
from a surface. The interested reader is referred to recent
extensive reviews of quats and polyquats as biocidal
materials
1,2
and an exhaustive patent literature.
3
A relatively new type of biocide, which will soon be
in use in the public sector, is the heterocyclic
N-halamine. Molecules representative of this type of
biocide contain either nitrogen– chlorine or nitrogen–
bromine covalent chemical bonds. They may be pre-
pared either as water-soluble monomers
4
or as water-
insoluble polymers.
2
If derivatized with electron-do-
nating alkyl groups adjacent to the nitrogen(s) on the
heterocyclic rings, the molecules will be very stable
toward release of free halogen into aqueous solution
and function as biocides by the direct contact of the
cells of microorganisms with the halogen atom. Fol-
lowing transfer of the oxidative halogen atom to the
cell, inactivation most probably proceeds by an oxida-
tion mechanism, as is presumed to be the case with
free available halogen (e.g., as in hypochlorite bleach).
Advantages inherent in the N-halamines as biocides
are the capability of regeneration following loss of the
halogen by simply exposing the molecules to addi-
tional free halogen, and, in general, more rapid inac-
tivation of a broad spectrum of pathogens than is the
case for quats and polyquats because oxidative chlo-
rine and bromine are potent biocides. Their primary
limitation is that being relatively new, some regula-
tory hurdles remain to be surmounted.
Correspondence to: S. D. Worley (worlesd@auburn.edu).
Contract grant sponsor: U.S. Air Force; contract grant
number: F08637-02-C-7020.
Contract grant sponsor: Vanson-HaloSource Corp.
Journal of Applied Polymer Science, Vol. 92, 363–367 (2004)
© 2004 Wiley Periodicals, Inc.