ISSN 1063-7834, Physics of the Solid State, 2009, Vol. 51, No. 3, pp. 507–513. © Pleiades Publishing, Ltd., 2009.
Original Russian Text © V.G. Zavodinsky, A.N. Chibisov, 2009, published in Fizika Tverdogo Tela, 2009, Vol. 51, No. 3, pp. 477–482.
507
1. INTRODUCTION
Among three crystalline forms of the titanium diox-
ide (rutile, anatase, brookite), the anatase has attracted
considerable attention of researchers owing to the
extensive applications as a catalyst, a component of
solar cells, and a coloring pigment. The TiO
2
dioxide
possessing a large reflection coefficient has been
widely used for protecting space vehicles against solar
radiation. However, in this case, the important factor is
the resistance of the coating with respect to the forma-
tion of color centers, which in the titanium dioxide are
predominantly represented by oxygen vacancies. In
recent years, investigations have been aimed at devel-
oping technologies that make it possible to increase the
radiation resistance of coatings based on the TiO
2
ana-
tase. For this purpose, the introduction of metal impuri-
ties into the titanium dioxide is one of the promising
directions. In particular, Mikhaœlov et al. [1] showed
that the introduction of silicon at small doses increases
the reflection coefficient, the addition of magnesium
decreases the reflection coefficient, and the simulta-
neous doping with magnesium and zinc increases the
radiation resistance. It should be noted that an increase
in the concentration of all these elements (from 0.5 to
1.0%) leads to a decrease in the reflection coefficient
and a deterioration of the radiation resistance. The
mechanism of the influence of these impurities on the
properties of the titanium dioxide remains unclear and
requires detailed investigations, including with the use
of theoretical approaches. The present study was
devoted to the solution of this problem.
2. CALCULATION METHOD
The introduction of impurities and the formation of
vacancies in the TiO
2
dioxide are frequently accompa-
nied by the spin polarization. Therefore, the total
energy and the electronic structure were calculated with
the FH196spin program package, which is a modifica-
tion of the FH196md program package [2] previously
used with advantage for many systems, including tran-
sition metal oxides [3–5]. This program package is
based on the spin-unrestricted version of the electron-
density functional theory, the pseudopotential method,
and the use of a plane-wave basis set. In this work, we
used the pseudopotentials of titanium and oxygen that
were constructed with the FHI98PP program package
[6]. The pseudopotentials were checked for the absence
of the so-called ghost states and used for determining
the equilibrium lattice parameters and the bulk elastic
modulus of the anatase. These pseudopotentials are
separable, transferable, and norm-conserving pseudo-
potentials [6]. The calculated values of the lattice
parameters and the elastic modulus differed from the
experimental values by no more than 2 and 10%,
respectively. A similar procedure was used for choosing
the pseudopotentials of impurity atoms. In all cases
(except for titanium), the pseudopotentials were calcu-
lated using the Troullier–Martins scheme [7]. For tita-
nium, the s and p components were determined accord-
ing to the Hamann technique [8] and the d component
was calculated within the Troullier–Martins scheme.
The parameters of the pseudopotentials used are listed
in Table 1.
Influence of Impurities on the Stability and Electronic States
of Titanium Dioxide in the Form of Anatase
V. G. Zavodinsky
a,
* and A. N. Chibisov
b,
**
a
Institute of Materials Science, Far East Division, Russian Academy of Sciences,
ul. Tikhookeanskaya 153, Khabarovsk, 680042 Russia
* e-mail: vzavod@mail.ru
b
Institute of Geology and Nature Management, Far East Division, Russian Academy of Sciences, Relochnyi per. 1,
Blagoveshchensk, 675000 Russia
** e-mail: andreichibisov@yandex.ru
Received July 16, 2008
Abstract—The behavior of impurities (Si, Zr, Mg, Zn) in the titanium dioxide with an anatase structure is
investigated using the electron-density functional method (with due regard for the spin polarization). The influ-
ence of these impurities on the formation of oxygen vacancies and the specific features of the electronic struc-
ture is studied. It is demonstrated that the impurities can both improve and deteriorate the optical characteristics
of the titanium dioxide.
PACS numbers: 71.15.Mb, 71.20.-b
DOI: 10.1134/S1063783409030123
1
DEFECTS AND IMPURITY CENTERS, DISLOCATIONS,
AND PHYSICS OF STRENGTH