RESEARCH ARTICLE
EXPERIMENTAL AND THEORETICAL STUDIES ON THE CORROSION INHIBITIVE PROPERTIES OF MILD
STEEL IN 2M H2SO4 ACID SOLUTION BY ETHANOLIC EXTRACT OF BRACHYSTEGIA EURYCOMA SEED
Chimezie P. Ozoemena
1
*, Milam Charles
2
, and Mary C. Ugwuoke
3
1
Department of Chemistry, University of Uyo, Akwa Ibom State, Nigeria
2
Department of Chemistry, Moddibo Adama University of Technology, Adamawa State, Nigeria
3
Department of Biochemistry, Michael Okpara Univsrsity of Agriculrure,Umudike, Abia State, Nigeria
ARTICLE INFO ABSTRACT
The experimental aspect of the corrosion inhibition potentials of Brachystegia eurycoma seed extract
was carried out using Phytochemical Screening and gravimetric techniques as well as scanning electron
microscopy (SEM) and Fourier transform infrared spectroscopy (FTIR), whereas the theoretical aspect
was studied using the density functional theory calculations to be performed and modeling the
electronic structures of some extract constituents, including physiosorptive interactions with the mild
steel surface. The analysis of the weight loss results showed that the Inhibition efficiency of the
Brachystegia eurycoma seed extract is directly proportional to its concentration and inversely
proportional to solution temperature and mild steel contact time in the test solution. The inhibition
efficiency increases gradually reaching a maximum value of 96% within the first 24 hours at a
concentration of 0.5g/l. The kinetic study shows that the inhibitory action is a first order kinetics with
the concentration of the seed extract of Brachystegia eurycoma which is best fitted with the Langmuir
adsorption isotherm. This was further supported by the thermodynamic parameters which indicate that
the adsorption of Brachystegia eurycoma seed extract onto the metal surface was spontaneous,
exothermic and has contributed to physical adsorption process. FTIR results showed that the inhibition
mechanism was an absorption process through the functional groups present in the seed extract. Surface
morphology also revealed that corrosion product confirmed the protection offered by the extract on the
surface of the metal immersed in the acid media. Quantum chemical studies indicated that inhibition
was due to adsorption of active molecules leading to formation of a protective layer on surface of mild
steel. Quantum chemical parameters such as highest occupied molecular orbital (HOMO), lowest
unoccupied molecular orbital (LUMO) energy levels, HOMO–LUMO energy gap and electronic
density were virtually identified. Quantum analysis demonstrated reactive centres of electrophilic and
nucleophilic attack and strong inhibition properties of bioactive molecules of BES extract.
Copyright © 2019, Chimezie P. Ozoemena et al. This is an open access article distributed under the Creative Commons Attribution License, which permits
unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
INTRODUCTION
The use of mild steel and any other metals in chemical
industries cannot be overstressed due to its mechanical
properties and wide range of application as structural material
for vessels reactor, pipelines, tank, construction works and
other industrial equipment which are known to corrode
invariably in contact with various solvents (S. Junaedi et al.,
2012). Acid solutions especially sulfuric acid used for
industrial processes such as acid pickling, industrial cleaning,
acid descaling, etching of metal and acidic operations may
cause damage to metal surface (Akalezi et al., 2012;
Okorokwo et al., 2015; Peter et al., 2016; Akalezi and Oguzie,
2015).
*Corresponding author: Chimezie P. Ozoemena,
Department of Chemistry, University of Uyo, Akwa Ibom State,
Nigeria.
However, contact between the metal and acidic media exposed
most industrial equipment to corrosion. Corrosion degrades the
useful properties of materials and structures including strength,
appearance and permeability to liquids and gases thereby
affecting the tensile strength and utility efficiency of the
material (Samuel et al., 2015). In view of the nation’s
economy and financial implications of corrosion menace,
researchers are compelled to do copious scientific studies in an
attempt to improve the resistance of metals. Corrosion
inhibitors have proven to be the most convenient means of
protecting metals due to their unique properties which
enhances their capability to resist the corrosion process as
compared to other methods (i.e. electroplating, coatings,
alloying elements, and plastic deformation) (U. Leon-Silva et
al., 2010; Gutierrez et al., 2016; EL-Basiony et al., 2019).
ISSN: 0976-3376
Asian Journal of Science and Technology
Vol. 10, Issue, 12, pp.10532-10544, December, 2019
Available Online at http://www.journalajst.com
ASIAN JOURNAL OF
SCIENCE AND TECHNOLOGY
Article History:
Received 15
th
September, 2019
Received in revised form
29
th
October, 2019
Accepted 17
th
November, 2019
Published online 30
th
December, 2019
Key words:
Corrosion, Corrosion Inhibitors, Mild
Steel, Weight Loss, scanning electron
microscopy, Quantum Analysis,
Kinetic, Thermodynamics.
Citation: Chimezie P. Ozoemena, Milam Charles and Mary C. Ugwuoke. 2019. “Experimental and Theoretical Studies on the Corrosion Inhibitive Properties of
mild Steel in 2M H2SO4 Acid Solution by Ethanolic Extract of Brachystegia Eurycoma Seed”, Asian Journal of Science and Technology, 10, (12), 10532-10544.