ORIENTAL JOURNAL OF CHEMISTRY
www.orientjchem.org
An International Open Access, Peer Reviewed Research Journal
ISSN: 0970-020 X
CODEN: OJCHEG
2020, Vol. 36, No.(6):
Pg. 1066-1077
This is an Open Access article licensed under a Creative Commons license: Attribution 4.0 International (CC- BY).
Published by Oriental Scientific Publishing Company © 2018
Spectrophotometric Determination of Low Levels of the
Orthophosphate Anion as Molybdenum Blue using Sodium
Thiosulphate Reducing agent
IRENE NALUMANSI
1
*, GRACE BIRUNGI
1
, BRENDA MOODLEY
2
and EMMANUEL TEBANDEKE
3
1
Department of Chemistry, Mbarara University of Science and Technology, Uganda.
2
School of Chemistry and Physics, University of Kwa Zulu-Natal, Westville Campus, South Africa.
3
Department of Chemistry, Makerere University, Uganda.
*Corresponding author E-mail: inalumansi@must.ac.ug
http://dx.doi.org/10.13005/ojc/360608
(Received: November 10, 2020; Accepted: December 11, 2020)
ABSTRACT
A simple spectrophotometric method for the determination of low levels of the orthophosphate
(PO
4
3-
) in environmental water systems is reported. The method is based the formation of the
phosphomolybdate from the condensation of molybdate and orthophosphate in aqueous acid medium
followed by reduction with sodium thiosulphate to form phosphomolybdenum blue. The system obeys
Beer’s law at 880 nm (λ
max
) in the 0.005–0.06 mg P mL
-1
phosphate concentration range. Molar absorptivity,
Sandell’s sensitivity and correlation coefficient values for the determination were 57526 L mol
-1
cm
-1
, 0.2835
μg cm
-2
and 0.9948 respectively. The limit of detection was 2.213 x 10
-3
mg P mL
-1
. The results of PO
4
3-
determination in water samples obtained using the spectrophotometric method developed in this study,
compare favourably with those generated using the Murphy and Riley method which is commonly used
for this analysis. Therefore, the study ably demonstrates the suitability of the present spectrophotometric
method for analysis of the orthophosphate in environmental water samples.
Keywords: Spectrophotometric, Phosphomolybdate, Molybdenum blue,
Orthophosphate anion, Sodium thiosulphate
INTRODUCTION
Phosphorus (P) a vital nutrient to human,
animal and plant growth occurs naturally in rocks and
soils as phosphorite or hydroxyapatite, Ca
3
(PO
4
)
2
.
Ca(OH)
2
, apatite, Ca
3
(PO
4
)
2
.CaF
2
, vivianite,
Fe
3
(PO
4
)
2
.8H
2
O and aluminium phosphate
1
. Since P
serves as a nutrient in the food chain, supplementing
the native P in the soil and animals’ diet where it is
lacking may be a necessity. This can result in excess
P moving from agricultural areas especially where
animal wastes are being used as fertilisers to other
environmental systems
2
. These phosphates stimulate
the growth of phytoplankton and aquatic plants
which provide food for many organisms including
zooplanktons, fish, humans and other mammals.
This may result in eutrophication of waters and its
related effects of anoxic conditions
3,4,5
; which leads to