1863 small 2010, 6, No. 17, 1863–1867 © 2010 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
Heterostructures
DOI: 10.1002/smll.200902348
Recent developments in the field of thin-film growth tech-
nologies have allowed control at an atomic level of deposited
layers, thus opening new perspectives in the field of engi-
neering of multilayers and heterostructures based on complex
oxides.
[1]
In particular, it is expected that oxide heterostruc-
tures, with almost ideal interfaces, may lead to interesting
artificial materials with novel properties. Artificial thin-film
oxide structures make the already complex individual bulk
properties even more interesting through their interaction at
the interface. Following such an approach, a number of het-
erostructures have been tailored which show extraordinary
properties that do not belong to the individual layers. These
range from superconductivity at the interface between non-
superconducting layers to high-mobility 2D conductivity at
the interface between insulating oxides.
[2,3]
The number of
possible combinations of these oxides is enormous, and the
potential for novel behavior having practical applications
represents a strong motivation for this research.
The same approach can be applied to heterostructures
based on oxide ionic conductors provided that the issues
concerning structural match at the interface are solved. The
interest in heterostructures based on oxide ionic conductors
is driven by the space-charge-zone effects at the interface,
which can increase the charge-carrier concentration locally,
and by interface mobility effects, the latter being of particular
relevance in the case of materials with high defect density
and relatively low mobility. The potential impact of oxide
ionic conductor superlattices has been shown for superlattices
based on CaF
2
and BaF
2
layers, grown by molecular beam
epitaxy, which exhibited an increase in ionic conductivity
Enhancement of Ionic Conductivity in Sm-Doped Ceria/
Yttria-Stabilized Zirconia Heteroepitaxial Structures
Simone Sanna, Vincenzo Esposito, Antonello Tebano, Silvia Licoccia,
Enrico Traversa,* and Giuseppe Balestrino*
with increasing number of interfaces.
[4]
For the thinner indi-
vidual layers, the conductivity increase of the superlattices
was up to two orders of magnitude larger than the conduc-
tivity of BaF
2
films over the whole measured temperature
range. These results were found to be in excellent agreement
with a model based on fluoride atom redistribution at the
interface. More recently, superlattices made of SrTiO
3
(STO)
and ZrO
2
:8 mol% Y
2
O
3
(yttria-stabilized zirconia, YSZ)
layers were investigated, and showed a colossal enhancement
of ionic conductivity, which was several orders of magnitude
larger than the YSZ conductivity, even at room tempera-
ture.
[5]
However, these findings were successively questioned
because the researchers omitted to consider the ionic and
electronic conductivity contribution from the much thicker
STO substrates they used.
[6]
To gain further insight into these findings, herein we
investigate the electrochemical properties of superlattices
made of alternate layers of 20 mol% samarium-doped ceria
(Ce
0.8
Sm
0.2
O
2- δ
, SDC) and 8 mol% YSZ, fabricated by pulsed
laser deposition (PLD). The choice of coupling SDC and
YSZ aimed to have both layers in the superlattices made
of oxygen-ion conductors with compatible crystallographic
features. These materials are highly defective, so that even-
tual interface effects are expected to be related to mobility
enhancement phenomena rather than to space-charge-region
effects.
[7]
SDC has a larger ionic conductivity than YSZ, the
conventional solid oxide fuel cell (SOFC) electrolyte mate-
rial, and is thus intensively studied to reduce the SOFC
operating temperature in the 600–800 °C range.
[8–10]
Several
superlattice films were prepared by varying the number of
SDC/YSZ bilayers N, keeping the same total thickness, and
the superlattice modulation length Λ (the thickness of an
individual SDC/YSZ bilayer), keeping the number of inter-
faces constant. Electrochemical measurements showed a size-
able increase in conductivity with increasing number of SDC/
YSZ interfaces, which does not have an electronic origin as
demonstrated by measurements at low oxygen partial pres-
sure ( pO
2
). The conductivity enhancement is attributed to
interfacial tensile strain effects rather than to interface space-
charge regions, due to the presence of a large defect concen-
tration in SDC and YSZ compounds.
Doped ceria films having a fluorite structure can be
deposited on several non-fluorite substrates by PLD, starting
from a polycrystalline target and maintaining the correct stoi-
chiometry.
[11]
In particular, doped ceria has been shown to
grow on (001) MgO substrates as well as on (001) LaAlO
3
Dr. S. Sanna, Dr. V. Esposito, Prof. S. Licoccia, Prof. E. Traversa
NAST Center & Department of Chemical Science and Technology
University of Rome Tor Vergata
Via della Ricerca Scientifica, 00133 Rome, Italy
E-mail: traversa@uniroma2.it
Dr. A. Tebano, Prof. G. Balestrino
CNR-SPIN & Department of Mechanical Engineering
University of Rome Tor Vergata
Via del Politecnico, 00133 Rome, Italy
E-mail: giuseppe.balestrino@uniroma2.it
Prof. E. Traversa
International Research Center for Materials Nanoarchitectonics (MANA)
National Institute for Materials Science (NIMS), 1–1 Namiki
Tsukuba, Ibaraki 305-0044, Japan