Journal of Encapsulation and Adsorption Sciences, 2018, 8, 39-57
http://www.scirp.org/journal/jeas
ISSN Online: 2161-4873
ISSN Print: 2161-4865
Adsorption Kinetics and Thermodynamics
Study of Butylparaben on Activated Carbon
Coconut Based
Patrick Atheba
1,2
, N’Guadi Blaise Allou
3*
, Patrick Drogui
1
, Albert Trokourey
2
1
Institut National de la Recherche Scientifique (INRS-ETE), Université du Québec, Quebec City, Canada
2
Laboratoire de Chimie Physique, Université Félix Houphouët Boigny de Cocody-Abidjan, Abidjan, Côte d’Ivoire
3
Advanced Materials Group, Materials Science and Technology Division, CSIR-NEIST, Jorhat, India
Abstract
In this work, low cost coconut biochar based activated carbon (CBAC) was
used for adsorption of Butylparaben (BPB) from aqueous medium. The pre-
pared CBAC was characterized using BET, Boehm analysis and the adsorption
equilibrium, kinetics and thermodynamics studies of BPB adsorption were
carried out. During batch adsorption runs, the effects of factors, such as con-
tact time (0 - 300 min), CBAC dose (200 - 800 mg), pH (3 - 11) and solution
temperatures (303 - 348 K) were investigated on BPB removal. Experimental
results reveal that the BPB removal efficiency on CBAC is higher than 97%
under acidic and neutral conditions. Equilibrium data were fitted by Lang-
muir, Freundlich and Temkin isotherm models with correlation coefficient
more than 0.9. The pseudo-second order kinetic model was observed to fit
well the adsorption data. Thermodynamic analysis shows positive values of
standard Gibb’s free energy, suggesting the non-spontaneity of the process.
The changes in enthalpy (0.2 J·mol
−1
) and entropy (19 J·mol
−1
) were found to
be endothermic with an increase of randomness. The high adsorption effi-
ciency of the synthesized coconut biochar materials with low cost indicates
that it may be a promising adsorbent for removing organic compounds.
Keywords
Coconut Shell, Activated Carbon, Adsorption, Butylparaben, Kinetics,
Isotherm
1. Introduction
During these last 20 years, concerns about the consequences of human and wild-
How to cite this paper: Atheba, P., Allou,
N.B., Drogui, P. and Trokourey, A. (2018)
Adsorption Kinetics and Thermodynamics
Study of Butylparaben on Activated Carbon
Coconut Based. Journal of Encapsulation
and Adsorption Sciences, 8, 39-57.
https://doi.org/10.4236/jeas.2018.82003
Received: February 6, 2018
Accepted: May 28, 2018
Published: May 31, 2018
Copyright © 2018 by authors and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access
DOI: 10.4236/jeas.2018.82003 May 31, 2018 39 Journal of Encapsulation and Adsorption Sciences