105
Bulgarian Chemical Communications, Volume 45, Special Issue B (pp. 105-109) 2013
XPS investigation on the surface of ZnO photocatalytic films obtained by polymer
modified spray pyrolysis
M. G. Shipochka
*
, I. D. Stambolova, V. N. Blaskov, P. K. Stefanov
Institute of General and Inorganic Chemistry, Bulgarian Academy of Sciences,
Acad. G. Bonchev St., bl.11, 1113 Sofia, Bulgaria.
Received October 17, 2013; Revised November 25, 2013
Photocatalytically active ZnO nanosized films were deposited by polymer modified spray pyrolysis method. The
influence of the polymers and the type of zinc precursor on the chemical composition, surface morphologies and the
photocatalytic properties towards Malachite Green dye degradation were investigated. The amount of oxygen in the
lattice (O
L
) and oxygen total (O
T
) as well as the atomic ratio of Zn/O
T
were evaluated by means of X-ray Photoelectron
Spectroscopy (XPS). The ZnO films are non-stoichiometric. The addition of polymers to both zinc salt solutions does
not change significantly the oxygen concentration in the films. After photocatalytic test the ratio O
L
/O
T
decreases,
showing that the amount of adsorbed hydroxyl groups is increased.
The films obtained from zinc acetate possess higher photocatalytic activity than those, obtained from zinc nitrate.
The highest efficiency is achieved with the films obtained from zinc acetate with ethylcellulose addition.
Keywords: ZnO, thin films, XPS surface analysis, spray pyrolysis, photocatalytic properties
INTRODUCTION
The growth of the world’s industry and
population has increased the demand for water
supply. The textile industries are among the
industries that consume largest volumes of water in
the processing operations including pre-treatment,
dyeing, pattern printing and finishing. It has been
reported that some of the dyes used in this industry
are toxic, mutagenic and carcinogenic [1]. In
general, photocatalysis is used as a pre-treating step
to degrade non-biodegradable organic pollutants to
biodegradable compounds. As a well-known
photocatalyst, ZnO has received much attention in
the degradation and complete mineralization of
environmental pollutants [2].
The spray pyrolysis process, as a simple and
easy thin films deposition method is one of the
versatile methods to prepare thin nanosize films.
The studies on the ZnO sprayed films surface by
XPS analysis before and after pfotocatalysis are
quite scarce in the available literature. This
information is important because it elucidates the
changes on the surface of the photocatalysts. Data
about the effects of the polymeric modifier, added
to the spray solution composition, and the nature of
the zinc precursor in regard to the effectiveness of
tuning of some physicochemical characteristics of
the ZnO films and their correlations with the
catalysts efficiency are quite a few.
In this paper we aimed at obtaining
correlations between the type of polymer additive
in the zinc precursor spray solution, some
physicochemical characteristics and the
photocatalytic properties of the ZnO films.
EXPERIMENTS
Two types of zinc precursor solutions have
been prepared for the purpose of spray pyrolysis
deposition. Zinc acetate (Zn(CH
3
COO)
2
) and zinc
nitrate (Zn(NO
3
)
2
) were diluted in an ethanol–water
mixture to obtain 0.4 M/L solutions of Zn and these
were denoted as “sol A” and “sol B”, respectively.
The ethanol-water volume ratio in the solutions was
3:1. Polyvinyl alcohol (PVA) was prepared in
ethanol-water mixture under stirring (sol C). A
defined quantity of “sol C” was added to sols A or
B in order to prepare the final spray solutions with
30 wt% PVA. The obtained solutions were denoted
as “sol AC” and “sol BC”, respectively. In parallel
to this the solution of ethyl cellulose
[C
6
H
7
O
2
(OC
2
H
5
)
3
]
n
in ethanol was prepared under
stirring for 2h (sol D) (40wt%) and then added to
“sol A” and “sol B” in order to obtain the final
solutions “sol AD” and “sol BD”. The aerosol was
transported to the aluminum foil plates heated at
© 2013 Bulgarian Academy of Sciences, Union of Chemists in Bulgaria
* To whom all correspondence should be sent:
E-mail: shipochka@svr.igic.bas.bg