Journal of Modern Physics, 2017, 8, 770-785
http://www.scirp.org/journal/jmp
ISSN Online: 2153-120X
ISSN Print: 2153-1196
DOI: 10.4236/jmp.2017.85049 April 25, 2017
Nitrogen Desorption and Positron Sensitive
Defect of CVD Diamond
Kasey R. Lund
1
, Kelvin G. Lynn
2
, Marc H. Weber
3
, Chao Liu
4
, Elgin Eissler
4
1
National Superconducting Cyclotron Laboratory Michigan State University, East Lansing, MI, USA
2
Center for Materials Research, Department of Physics, School of Mechanical and Materials Engineering, Washington State
University, Pullman, WA, USA
3
Center for Materials Research, Washington State University, Pullman, WA, USA
4
II-VI Incorporated, Saxonburg, PA, USA
Abstract
The chemical vapor deposition (CVD) process can produce single or poly-
crystalline diamond samples of high purity or with controlled doping concen-
trations. The defect type in the CVD diamonds can be changed by heating the
samples. Controlling the defect type can be used to create devices for quantum
diamond switches that could be used in radiation sensors and quantum in-
formation technology. Eight samples of CVD diamonds were analyzed with
Doppler broadening of positron annihilation radiation (DBAR) before and
after annealing in high vacuum with an electron gun. Between temperatures
of 1700 - 1850 K, nitrogen was liberated from the diamond sample. At these
high temperatures, the surface was graphitized and a change in the color and
transparency of the diamond was observed. Some of the samples were ana-
lyzed with DBAR during periods with and without light. The defect properties
were observed to change depending on the time exposure to the positron
beam and were then regenerated by exposure to light. The DBAR data is
compared to photoluminescence data and a time varying defect state is dis-
cussed for detector and optical grade type II CVD diamonds.
Keywords
CVD Diamond Detectors, Positron Annihilation Spectroscopy, Divacancy
1. Introduction
Much attention has been giving to CVD diamonds because of their electrical and
mechanical properties. Previous work [1] [2] [3] has shown that CVD diamonds
can be manipulated to tune their properties in order to create devices for quan-
tum mechanical diamond switches that could be used in diamond sensors, io-
How to cite this paper: Lund, K.R., Lynn,
K.G., Weber, M.H., Liu, C. and Eissler, E.
(2017) Nitrogen Desorption and Positron
Sensitive Defect of CVD Diamond. Journal
of Modern Physics, 8, 770-785.
https://doi.org/10.4236/jmp.2017.85049
Received: March 9, 2017
Accepted: April 22, 2017
Published: April 25, 2017
Copyright © 2017 by authors and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access