Research Article
Synthesis of Poly-(R-hydroxyalkanoates) by
Cupriavidus necator ATCC 17699 Using Mexican Avocado
(Persea americana) Oil as a Carbon Source
Araceli Flores-Sánchez,
1
Ma. del Rocío López-Cuellar,
2
Fermín Pérez-Guevara,
3
Ulises Figueroa López,
1
José Mauricio Martín-Bufájer,
1
and Berenice Vergara-Porras
1
1
Escuela de Ingenier´ ıa y Ciencias, Tecnol´ ogico de Monterrey, Campus Estado de M´ exico, Carretera Lago de Guadalupe Km 3.5,
Margarita Maza de Ju´ arez, Atizap´ an de Zaragoza, MEX, Mexico
2
Cuerpo Academico de Biotecnolog´ ıa Agroalimentaria, Instituto de Ciencias Agropecuarias, Universidad Aut´ onoma del Estado de
Hidalgo, Pachuca, HGO, Mexico
3
Departamento de Biotecnolog´ ıa y Bioingenier´ ıa, Centro de Investigaci´ on y Estudios Avanzados (CINVESTAV), Avenida IPN 2508,
Zacatenco, Gustavo A. Madero, Ciudad de M´ exico, Mexico
Correspondence should be addressed to Berenice Vergara-Porras; vergarabp@itesm.mx
Received 20 April 2017; Accepted 14 June 2017; Published 21 August 2017
Academic Editor: Rafaele Cucciniello
Copyright © 2017 Araceli Flores-S´ anchez et al. Tis is an open access article distributed under the Creative Commons Attribution
License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly
cited.
Poly-R-hydroxyalkanoates (PHAs) are polymers produced by a vast number of bacterial species under stress conditions. PHAs
exhibit diferent thermal and mechanical properties that depend on their molecular structure. In this work, PHAs were produced
using avocado oil as the carbon source. Cupriavidus necator H16 was cultured in three-stage fermentation using fructose during
the cell growth stages and avocado oil during the PHA synthesis stage. Diferent concentrations of avocado oil were used during
the third stage to test the incorporation of various monomeric units into the PHAs. Biomass and PHA production were measured
during the fermentation. DSC, FTIR, and gas chromatography analysis aided the PHA characterization. Diferent proportions of
3-hydroxyvalerate were present in the 3-hydroxybutyrate main chain depending on the concentration of avocado oil. Te results
suggest that avocado oil is a viable new substrate for PHA production.
1. Introduction
Poly-R-hydroxyalkanoates (PHAs) are polymers synthesized
by a large number of bacterial species as a response to
unbalanced nutritional conditions [1]. PHAs are thermoplas-
tic polyesters of R-hydroxy alkanoic acids and accumulate
intracellularly as granules that exhibit diferent properties
depending on their chemical composition [2, 3]. A single
monomer that forms the chain of PHAs typically contains
from 3 to 15 carbon atoms [4], but the fnal chemical compo-
sition of PHAs is related to the synthesizer microorganism,
the carbon source, the culture conditions, and the specifcity
of the PHA-synthase enzyme [5–7]. Homopolymers, copoly-
mers, or terpolymers of PHAs can be obtained; for example,
PHA copolymers can be synthesized from a combination of
diferent substrates [8]. Te thermal properties of PHAs, such
as melting temperature and degree of crystallinity, depend
on the length of the PHA monomeric units. Monomers con-
taining more than fve carbon atoms signifcantly decrease
the polymer melting temperature, as well as the degree of
crystallinity [9].
Many PHAs have main chains formed from monomers
with diferent numbers of carbon atoms. Short-length-chain
PHAs (PHA
slc
) consist of monomers ranging from 3 to 5
carbons, whereas medium-length-chain PHAs (PHA
mlc
) are
formed from monomers containing 6 to 14 carbon atoms
[4, 8]. One PHA
slc
, poly(3-hydroxybutyrate) (PHB), is the
most common PHA and was frst identifed by Maurice
Lemoigne in 1926 [1, 4]. PHB biodegradability and bio-
compatibility make it an attractive material; however, its
Hindawi
International Journal of Polymer Science
Volume 2017, Article ID 6942950, 10 pages
https://doi.org/10.1155/2017/6942950