Vietnam Journal of Chemistry, 2018, 56(4), 473-477 Article
DOI: 10.1002/vjch.201800032
473 Wiley Online Library © 2018 Vietnam Academy of Science and Technology, Hanoi & Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
Bismuth nanodendrites deposited on glassy carbon electrode as a
sensitive electrochemical sensor for simultaneous detection of
Cd
2+
and Pd
2+
ions
Nguyen Hoang Anh
1
, Pham Khac Duy
1
, Pham Thi Hai Yen
1
, Vu Hai Dang
1
,
Nguyen Quynh Giao
1
, Vu Thi Thu Ha
1,2*
1
Institute of Chemistry, Vietnam Academy of Science and Technology (VAST), 18 Hoang Quoc Viet, Cau
Giay district, Hanoi 100000, Viet Nam
2
University of Science and Technology of Hanoi (USTH), VAST, 18 Hoang Quoc Viet, Cau Giay district,
Hanoi 100000, Viet Nam
Received March 16
th
2018; Accepted for publication June 15
th
2018
Abstract
In this study, bismuth nanodendrites (BiNDs) were fabricated on glassy carbon electrode by
chronopotentiometric method. The hierarchical structure and high population matrix of BiNDs provides high surface
active area to enhance the electrochemical signals of measured Cd
2+
and Pb
2+
ions. The developed bismuth
nanodendritic structure was well-observed and characterzied by scanning electron microscopy (SEM).
Electrochemical behaviours of developed BiNDs electrodes were studied by the cyclic voltammetric (CV) method.
The fabrication conditions for BiNDs such as the applied current and deposition time were optimized as -10 mA
and 90 s, respectively. Under this optimized condition, the highest peaks of Cd
2+
and Pb
2+
ions at concentration of
20 ppb were obtained. The Cd
2+
and Pb
2+
signals acquired by BiNDs are almost three times greater than that
measured by the Bi film electrode.
Keywords. Bi nanodendrite, electrodeposition, surface structure, electrochemical behaviours, cadmium, lead.
1. INTRODUCTION
Recently, the electrochemical methods have been
strongly developed for simultaneous dectection of
heavy metals due to their good selectivity, high
accuracy, low expense of instrument, portability and
operation simplicity.
[1]
Among various
electrochemically analytical techniques, the anodic
stripping voltammetry (ASV) is commonly used
for determination of heavy metals at the same time
such as zinc, cadmium, lead and copper because of
its convenience not only in laboratory condition but
also on-site. The conventional working electrode
used in the method is mercury film electrodes due to
its good reproducibility and high sensitivity.
[2]
However, many alternative materials have been
found to replace mercury beacause of its extreme
toxicity of mercury to the environment and human
health. Bismuth electrode were first studied by J.
Wang in 2000 as the best replacement because of
similar electrochemical properties to mercury
electrode such as wide potential window; well-
defined, good signal-to-background characteristics;
forming fused multicomponent alloys with heavy
metals.
[1]
Especially, bismuth is a friendly-
environmental material which is employed in many
fields including catalysis, photonics, electronics,
optoelectronics, energy storage, sensor,
superconductive material even in pharmaceutical
products.
[3]
There are many modifications of bismuth on
different substrates in order to enhance the
electrochemical signals of the heavy metals. Among
them, bismuth film electrodes (BiFE) were widely
used.
[4,5]
The differrent forms of bismuth such as
nanoparticles, nano rods
[6]
and nanosheets,
[7]
microrods on glassy carbon and film were also well
studied.
[8]
Conventionally, the electrochemical
deposition method was applied; only few studies
reported the chemical method for the fabrication of
Bi nanostructure.
[9]
In this study, the bismuth nanodendrite was
succesfully obtained by chronopotentiometric
method. The electrodeposition condition of the
BiNDs was carefully examined. The obtained
BiNDs with hierarchical structure and high