148
Original article doi: 10.12980/jclm.4.2016j5-219 ©2016 by the Journal of Coastal Life Medicine. All rights reserved.
Sri Lankan black tea (Camellia sinensis L.) inhibits the methylglyoxal mediated protein glycation and
potentiates its reversing activity in vitro
Walimuni Kanchana Subhashini Mendis Abeysekera
1
, Chatura Tissa Dayendra Ratnasooriya
2
, Wanigasekara Daya Ratnasooriya
3
, Sirimal
Premakumara Galbada Arachchige
1*
1
Industrial Technology Institute (ITI), 363, Bauddhaloka Mawatha, Colombo 07, Sri Lanka
2
Faculty of Medicine, University of Colombo, Colombo 08, Sri Lanka
3
Department of Basic Sciences, Faculty of Allied Health Sciences, General Sir John Kotalawala Defense University, Ratmalana, Sri Lanka
Journal of Coastal Life Medicine 2016; 4(2): 148-153
Journal of Coastal Life Medicine
*Corresponding author: Sirimal Premakumara Galbada Arachchige, Industrial
Technology Institute, 363, Bauddhaloka Mawatha, Colombo 07, Sri Lanka.
Tel: +94-11-2379800
E-mail: gasp@iti.lk; dg@iti.lk
The journal implements double-blind peer review practiced by specially invited
international editorial board members.
1. Introduction
Glycation, non-enzymatic glycosylation of proteins by glucose
is a relatively slow and complex series of endogenous reactions
occurring in the body, giving rise to various different glycotoxins
which are known as advanced glycation end products (AGEs)
[1-5]. Accumulation of AGEs is now implicated as a major factor
in the pathogenesis of long term complications of diabetes such
as retinopathy, nephropathy and end stage renal disease[1-5].
AGEs are also linked to mechanisms responsible for development
and progression of non-diabetic nephropathy, macro-vascular
disease, cancer, rheumatic arthritis, osteoarthritis, atherosclerosis,
cataract, neurodegenerative diseases including Alzheimer’s disease,
Parkinson disease and amyotrophic lateral sclerosis and age-related
cognitive decline[2,4]. Further, the formation of AGEs is known to
progressively increase with normal ageing, even in the absence of
disease[4].
Low molecular weight carbonyl compounds such as glyoxal and
methylglyoxal (MGO), most importantly MGO behave as precursors
of AGEs[4-6]. They form adducts on proteins, inducing cellular
dysfunctions leading to long term diabetes complications and other
age related diseases[2,4-6]. Thus, pharmaceutical agents (natural and/
ARTICLE INFO ABSTRACT
Objective: To evaluate inhibitory activity of methylglyoxal (MGO) mediated protein glycation
and ability to potentiate its reversing activity and range of antioxidant properties of Sri Lankan
low grown orthodox orange pekoe grade black tea.
Methods: Freeze dried black tea brew (BTB) was used as the sample in this study. Anti-
glycation and glycation reversing activity was studied in bovine serum albumin (BSA)-MGO
model. Antioxidant properties were studied using total polyphenolic content, total flavonoid
content, 2,2’-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid, 1,1-diphenyl-2-picrylhydrazine
and ferric reducing antioxidant power in vitro antioxidant assays.
Results: The results demonstrated significant (P < 0.05) and dose dependant inhibition of
BSA-MGO glycation [IC
50
: (164.30 ± 4.85) µg/mL], potentiating of its reversing activity [EC
50
:
(235.39 ± 5.37) µg/mL] and marked antioxidant properties [total polyphenolic content: (119.55
± 9.97) mg gallic acid equivalents/g BTB; total flavonoid content: (6.04 ± 1.26) mg quercetin
equivalents/g BTB; 2,2’-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid, 1,1-diphenyl-2-
picrylhydrazine and ferric reducing antioxidant power: (3.29 ± 0.06), (1.95 ± 0.15) and (1.31
± 0.19) mmol Trolox equivalents/g BTB, respectively]. No correlations were observed between
antioxidant activity and BSA-MGO glycation.
Conclusions: The novel properties observed for Sri Lankan orange pekoe grade black tea
indicate its usefulness as a supplementary beverage in managing MGO and advanced glycation
end products related diseases and ailments.
Article history:
Received 5 Nov 2015
Received in revised form 4 Dec 2015
Accepted 22 Dec 2015
Available online 18 Jan 2016
Keywords:
Methylglyoxal
Advanced glycation end products
Glycation reversing
Diabetes complications
Orange pekoe grade black tea
Sri Lankan tea
journal homepage: www.jclmm.com