Research Article
Investigations into Recycling Zinc from Used Metal Oxide
Varistors via pH Selective Leaching: Characterization, Leaching,
and Residue Analysis
Toni Gutknecht,
1
Anna Gustafsson,
1
Christer Forsgren,
2
Christian Ekberg,
1
and Britt-Marie Steenari
1
1
Industrial Materials Recycling, Department of Chemical Engineering, Chalmers University of Technology,
Kemiv¨ agen 4, 412 96 Gothenburg, Sweden
2
Stena Metall AB, Fiskhamnsgatan 8D, Box 4088, 400 40 Gothenburg, Sweden
Correspondence should be addressed to Toni Gutknecht; tonig@chalmers.se
Received 12 May 2015; Accepted 5 August 2015
Academic Editor: Fernando Pelisser
Copyright © 2015 Toni Gutknecht et al. Tis is an open access article distributed under the Creative Commons Attribution License,
which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
Metal oxide varistors (MOVs) are a type of resistor with signifcantly nonlinear current-voltage characteristics commonly used in
power lines to protect against overvoltages. If a proper recycling plan is developed MOVs can be an excellent source of secondary
zinc because they contain over 90 weight percent zinc oxide. Te oxides of antimony, bismuth, and to a lesser degree cobalt,
manganese, and nickel are also present in varistors. Characterization of the MOV showed that cobalt, nickel, and manganese were
not present in the varistor material at concentrations greater than one weight percent. Tis investigation determined whether a pH
selective dissolution (leaching) process can be utilized as a starting point for hydrometallurgical recycling of the zinc in MOVs.
Tis investigation showed it was possible to selectively leach zinc from the MOV without coleaching of bismuth and antimony
by selecting a suitable pH, mainly higher than 3 for acids investigated. It was not possible to leach zinc without coleaching of
manganese, cobalt, and nickel. It can be concluded from results obtained with the acids used, acetic, hydrochloric, nitric, and
sulfuric, that sulfate leaching produced the most desirable results with respect to zinc leaching and it is also used extensively in
industrial zinc production.
1. Introduction
It is the vision for Europe to have market and policy incentives
in place by 2020 that will stimulate new innovations in
resource efcient production methods with all companies
being able to measure their lifecycle resource efciency [1].
It is with this vision that the importance of this work comes
to light. Electrical transmission and distribution equipment
such as insulators and protective equipment will become a
potentially large source of solid waste suitable for recycling as
opposed to landflling. Recycling of the used varistor mate-
rial and production waste promotes sustainable production
and consumption. Moreover, improving waste management
makes better use of resources while encouraging less depen-
dence on imports of raw material [1].
In Sweden, there is an initiative to recycle MOV as
opposed to landflling due to environmental concerns, rising
costs of landflling, awareness of the potential value of the
material in the MOV, and the quantity of material available
for recycling. In Sweden from 2009 to 2013 over 500 tons of
MOV was available for recycling [2]. However, a commercial
method for recycling of the MOV is not yet available and the
material is at the moment stored or landflled. If the ZnO was
purifed and converted to zinc metal the value of the metallic
zinc would be over $800,000 USD [3]. Te used varistors are
primarily not mixed with other types of waste materials but
kept in a separate fow which is a good starting point for a
recycling process. Te authors have not found any literature
on recycling of MOVs.
Hindawi Publishing Corporation
e Scientific World Journal
Volume 2015, Article ID 653219, 11 pages
http://dx.doi.org/10.1155/2015/653219