CHEMICAL ENGINEERING TRANSACTIONS
VOL. 80, 2020
A publication of
The Italian Association
of Chemical Engineering
Online at www.cetjournal.it
Guest Editors: Eliseo Maria Ranzi, Rubens Maciel Filho
Copyright © 2020, AIDIC Servizi S.r.l.
I SBN 978-88-95608-78-5; I SSN 2283-9216
Use of FTIR Spectroscopy and PLS-Regression in Monitoring
Biomolecules in Spirulina platensis during its Growth in an
Internally-Illuminated Photobioreactor
Butch G. Bataller
a,
*, Sergio C. Capareda
b
a
University of the Philippines Los Baños, Laguna, Philippines
b
Texas A&M University, Texas, USA
bgbataller@up.edu.ph
This study developed a rapid and non-destructive analytical method for biochemical analysis of the Spirulina
biomass via FTIR spectroscopy and PLS regression. It was then used to monitor the biochemical changes in
the biomass during an 8-day cultivation period in a 3-L internally-illuminated concentric-tube airlift
photobioreactor at different light intensities (69, 110, and 166 μmol photons m
-2
s
-1
). It was found that PLS-
regression have better predictive power than multipoint regression. It also yielded statistically similar results
with conventional biochemical methods. This new method reduced the time for sample preparation and
eliminated the extraction of target biomolecule for analysis. It was also found to be valuable in monitoring the
changes in the total protein, carbohydrate and lipid content (% w/w of total biomolecules) in Spirulina biomass
during its growth. It was observed that the protein content of the biomass decreased initially, which was
compensated by an increase in the carbohydrate content. This may imply that biomass production may be
driven by production of more carbohydrates during the early period of growth. Protein content then started to
increase until the third day of growth and remained constant thereafter. Carbohydrate and lipid content also
remained constant from the third day of growth. The lowest light intensity was found to have the highest
protein content (60.4± 0.87 %w/w) but it has the lowest overall biomass productivity (0.090 ± 0.017 g L
-1
d
-1
).
While at the highest light intensity, protein content was slightly lower (57.3 ± 0.777 %w/w) than that of the
lowest light intensity. But it has the highest overall biomass productivity (0.141 ±0.007 g L
-1
d
-1
).
1. Introduction
Conventional biochemical methods in quantifying biomolecules such as proteins, carbohydrates, and lipids in
algal biomass are usually time-consuming due to the series of steps that need to be undertaken during the
analysis. These steps usually require sample preparation and extraction steps before measurement can be
done. In extracting the target analyte, conventional biochemical methods often require high temperature that
may be destructive to the sample. For example, the proteins are extracted from the biomass at high
temperature using alkaline solution or a detergent-containing buffer. To prevent underestimation of protein
content, several extraction steps are necessary to ensure maximum extraction of protein. In carbohydrate
analysis via the phenol-sulfuric acid method, breaking down the polysaccharides and oligosaccharides to their
constituent monosaccharides often uses strong acids and often takes four hours in boiling water baths. These
methods also often require toxic and corrosive reagents that are harmful to human health and the
environment.
These methods are also sensitive to other interfering substances. For example, Lowry assay for protein
analysis is sensitive to the presence of carbohydrate, glycerol, and EDTA that are typically present in algal
extracts or in extraction buffers (Quiang and Richmond 2013). Detergents like sodium dodecyl sulfate and
Triton X-100 may also interfere with color development in Bradford protein assay. Overestimation of protein
may also result due to high presence of arginine and/or phenylalanine that bind disproportionately with the
Coomassie Brilliant Blue G250 dye (Quiang and Richmond 2013). Phenol-sulfuric acid method for
DOI: 10.3303/CET2080018
Paper Received: 13 November 2019; Revised: 3 February 2020; Accepted: 29 April 2020
Please cite this article as: Bataller B., Capareda S., 2020, Use of Ftir Spectroscopy and Pls-regression in Monitoring Biomolecules in Spirulina
Platensis During Its Growth in an Internally-illuminated Photobioreactor , Chemical Engineering Transactions, 80, 103-108
DOI:10.3303/CET2080018
103