International Journal of Thermophysics (2018) 39:94
https://doi.org/10.1007/s10765-018-2411-2
ICPPP 19
Fourier-Transform Infrared Differential Photoacoustic
Spectroscopy (FTIR-DPAS) for Simultaneous Monitoring
of Multiple Air Contaminants/Trace Gases
Lixian Liu
1,2
· Andreas Mandelis
1
· Huiting Huan
1
Received: 17 October 2017 / Accepted: 13 June 2018 / Published online: 22 June 2018
© Springer Science+Business Media, LLC, part of Springer Nature 2018
Abstract
Air pollutants have severe impact on the global environment and the health of human
beings. There is an urgent need for cost-effective devices for trace gas monitoring in
ambient conditions. However, water vapor in ambient air is still an obstacle in the
trace gas absorption detection field due to its complex and strong infrared absorb-
ing characteristics. In this work, a step-scan Fourier-transform infrared differential
photoacoustic spectroscopy (FTIR-DPAS) methodology developed in our laboratory
through the introduction of two identical T-resonators for enhancing and resolving
the DPA signal from two potentially pollutant gases is extended to multiple ambient
gas components: carbon dioxide (CO
2
) and acetylene (C
2
H
2
). A key feature of this
technique is the ability to resolve hidden target spectral components in ambient air:
Despite the fact that the acetylene absorption peaks lie within the strong water vapor
absorption band, the infrared PA absorption spectra of acetylene and carbon dioxide
are detected with high sensitivity and selectivity in the presence of significant interfer-
ence of water vapor in the laboratory ambient air, thereby confirming the superiority
and capability of step-scan FTIR-DPAS configuration to effectively and totally sup-
press often dominant background water signals and simultaneously detect multiple
trace gases.
Keywords Differential mode · FTIR-DPAS · Water vapor absorption cancelation
This article is part of the selected papers presented at the 19th International Conference on Photoacoustic
and Photothermal Phenomena.
B Andreas Mandelis
mandelis@mie.utoronto.ca
1
Center for Advanced Diffusion-Wave and Photoacoustic Technologies (CADIPT), Department of
Mechanical and Industrial Engineering, University of Toronto, Toronto, ON M5S 3G8, Canada
2
Present Address: School of Physics and Optoelectronic Engineering, Xidian
University, Xi’an 710071, China
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