177
Factors controlling major ion and trace element
content in surface water at Asprolakkas
hydrological basin, NE Chalkidiki:
Implications for elemental
transport mechanisms
E. Kelepertzis
1
, A. Argyraki, E. Daftsis
1
Corresponding author: Section of Economic Geology and Geochemistry, Faculty of
Geology and Geoenvironment, National and Kapodistrian University of Athens,
Panepistimiopolis, Zographou 157 84, e-mail: kelepert@geol.uoa.gr
Abstract Chemical characteristics of stream water at Asprolakkas hydrological
basin were determined in February 2009 in order to examine the main factors con-
trolling the hydrogeochemistry of the drainage system. A total of 20 surface water
samples were collected and analyzed for the major ions K, Na, Ca, Mg, HCO
3
,
SO
4
and the trace elements Fe, Pb, Zn, Mn, Cu, Ni, As, Sb, Mo and Ba. The appli-
cation of R-mode factor analysis revealed that the polymetallic carbonate re-
placement type sulfide deposits, together with the porphyritic intrusions and the
associated porphyry copper style mineralization, occurring in the studied area, im-
pose fundamental control on the water chemistry. A third influencing factor in-
cludes the parameters As and HCO
3
and is attributed to the competitive behavior
of As and bicarbonate ions, for filling in available absorption space on Fe(III) ox-
ides. SEM-EDS methods, performed on retained filters from the filtration of rep-
resentative water samples, showed that Pb is mainly transported by fine particulate
matter. The chemical elements Mn, Zn, Mo and Sb are predominantly present as
dissolved free ions, and correlate strongly with the electrical conductivity of the
water samples.
1 Introduction
Mineral deposit regional geology and geochemical processes are fundamental con-
trols on the surface water quality (Kelley and Taylor 1997). Apart from the very
mobile and bioavailable dissolved forms of trace metals, suspended particulate
matter and colloids are significant metal carrier phases. Colloids are particles that
have at least one dimension in the size range of 1-1000 nm, and due to their small
size they have a large specific surface area. These physical properties make col-
loids to have a significant impact on the transport of trace metals through sorption
N. Lambrakis et al. (Eds.), Advances in the Research of Aquatic Environment, Vol. 2
DOI 10.1007/978-3-642-24076-8, © Springer-Verlag Berlin Heidelberg 2011