Research Article
Distribution and Identification of Sources of Heavy Metals in
the Voghji River Basin Impacted by Mining Activities (Armenia)
A. V. Gabrielyan,
1
G. A. Shahnazaryan ,
1
and S. H. Minasyan
2
1
“Environmental Monitoring and Information Center” SNCO, 0012 Yerevan, Armenia
2
Institute of Chemical Physics, NAS RA, 0014 Yerevan, Armenia
Correspondence should be addressed to G. A. Shahnazaryan; gayane shahnazaryan@yahoo.com
Received 23 December 2017; Revised 11 February 2018; Accepted 18 February 2018; Published 18 March 2018
Academic Editor: Xiao-San Luo
Copyright © 2018 A. V. Gabrielyan et al. Tis is an open access article distributed under the Creative Commons Attribution License,
which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
Te objective of this research is to assess the distribution of heavy metals in the waters and sediments of the Voghji River and its
tributaries impacted by mining activity and to reveal the real source of each of the heavy metals in the environment for assessing
the pollution level of heavy metals. Voghji River with two main tributaries (Geghi and Norashenik) drain two mining regions. To
identify distribution and pollution sources of heavy metals, the water and sediment samples were collected from eight sampling sites.
Te results of statistical analysis based on data sets of the period 2014–2016 showed that, afer the infuence of drainage water and
wastewater of mining regions, heavy metal contents in the Voghji River basin dramatically increased. Te waters of the Voghji River
were highly polluted by Mn, Co, Cu, Zn, Mo, Cd, and Pb. Te relation of metals content was highly changed due to anthropogenic
impact disturbing the geochemical balance of the Voghji River. Te water quality based on only heavy metal contents in the source
of the Voghji River belongs to “good” chemical status, and in the sources of Geghi and Norashenik Rivers it is “moderate.” Te
water quality of Voghji and Norashenik Rivers is sharply worsening afer the infuence of mining activity, becoming “bad” chemical
status. Te research revealed the pollution sources of each metal.
1. Introduction
Impact of mining on aquatic ecosystems became an issue of
increasing concern. Mining by its nature consumes, diverts,
and seriously pollutes water resources [1–3]. Mining and
milling operations, together with grinding, concentrating
ores, and disposal of tailings, provide obvious sources of
contamination in the surface environment, along with dis-
charge or overfow of wastewater, runof from rainfall or
snowmelt, drainage from the toe of waste piles, and discharge
of impacted groundwater to streams and springs. Water
pollution problems caused by mining include acid mine
drainage, metal contamination, and increased sediment levels
in streams [4, 5]. Te generation of acidic drainage and
the release of water containing high concentrations of dis-
solved metals from mine wastes constitute an environmental
problem of international scale [6–8]. Chemical leaching of
metals occurs when precipitation from rainfall or snowmelt
infltrates through ore or waste materials and dissolves or
desorbs metals from the solid material. As a consequence,
streams transport high contents of toxic trace elements such
as As, Cd, Pb, Zn, Cu, Sb, and Se [9].
Heavy metals are an important class of pollutants which
can produce considerable harm to the environment when
they are above certain concentrations [10–12]. Tese elements
can be leached into the surface water or groundwater, taken
up by plants, and can bond semipermanently with soil
components such as clay or organic matter, which later afect
human health [13]. Afer heavy metals enter into a water
body, they can harm aquatic organisms, and, through the
processes of chemical adsorption and physical precipitation,
heavy metals can accumulate in the sediments of the water
environment [14]. Heavy metal contents of the surface sedi-
ments are generally signifcantly higher compared with those
in the water body, so it is very important to explore the heavy
metal contents in the surface sediments [15, 16].
Heavy metals are defned as metallic elements that have a
relatively high density compared to water. With the assump-
tion that heaviness and toxicity are interrelated, heavy metals
also include metalloids, such as arsenic, that are able to induce
Hindawi
Journal of Chemistry
Volume 2018, Article ID 7172426, 9 pages
https://doi.org/10.1155/2018/7172426