Jointly published by React.Kinet.Catal.Lett.
Akadémiai Kiadó, Budapest Vol. 80, No. 2, 375-381
and Kluwer Academic Publishers, Dordrecht (2003)
0133-1736/2003/US$ 20.00.
© Akadémiai Kiadó, Budapest.
All rights reserved.
RKCL4304
KINETICS OF METHANE COMBUSTION ON Fe
2
O
3
/TiO
2
CATALYSTS
Gina Pecchi
*
, Patricio Reyes and Raúl Zamora
Facultad de Ciencias Químicas, Universidad de Concepción, Casilla 160-C, Concepción, Chile
Received March 7, 2003
In revised form June 19, 2003
Accepted June 23, 2003
Abstract
The objective of this work was to study the kinetics of methane combustion for a
series of Fe
2
O
3
/TiO
2
catalysts. An increase in activity is observed as iron loading
increases, and can be attributed to an increase of surface coverage by Fe
2
O
3
species. Kinetic studies revealed that the reaction orders with respect to methane,
oxygen, carbon dioxide and water are 1, 0, 0 and –1 respectively.
Keywords: Iron, titania, combustion, methane
INTRODUCTION
Catalytic combustion is one of several industrial processes used for
pollution abatement. Catalysts able to perform combustion are divided in two
groups: noble metals and transition metal oxides. The noble metals, such as Pt
and Pd [1, 2], are more efficient because the reactions may start at temperatures
as low as room temperature, while transition metal oxides are less efficient but
more resistant at high temperatures. With regard to transition metal oxides their
low cost and availability as well as their interesting properties (e.g., good
activity as photocatalysts in the case of Fe and an increase in the stability in the
case of Cu) make them excellent candidates to rival noble metals [3]. The use
_______________________________________
*
Corresponding author